Unconventional spin dynamics and supersolid excitations in the triangular-lattice XXZ model

Motivated by recent experiments, we investigate the spin- <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:mfrac> <a:mn>1</a:mn> <a:mn>2</a:mn> </a:mfrac> </a:math> XXZ model on the triangular lattice with strong Ising anisotropy, combining large-scale numerical simulations and analytical methods to uncover unconventional spin dynamics at <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"> <b:mrow> <b:mi>T</b:mi> <b:mo>=</b:mo> <b:mn>0</b:mn> </b:mrow> </b:math> . First, we compute the dynamical spin structure factor using density matrix renormalization group (DMRG) simulations and find excellent agreement with inelastic neutron scattering data on the layered compound <c:math xmlns:c="http://www.w3.org/1998/Math/MathML"> <c:mrow> <c:msub> <c:mtext>K</c:mtext> <c:mn>2</c:mn> </c:msub> <c:mtext>Co</c:mtext> <c:msub> <c:mrow> <c:mo>(</c:mo> <c:msub> <c:mtext>SeO</c:mtext> <c:mn>3</c:mn> </c:msub> <c:mo>)</c:mo> </c:mrow> <c:mn>2</c:mn> </c:msub> </c:mrow> </c:math> . The low-energy spectrum reveals a rotonlike minimum at the <d:math xmlns:d="http://www.w3.org/1998/Math/MathML"> <d:mi>M</d:mi> </d:math> point, absent in linear spin-wave theory, accompanied by peak intensity and a broad continuum above it. Near the <e:math xmlns:e="http://www.w3.org/1998/Math/MathML"> <e:mi mathvariant="normal">Γ</e:mi> </e:math> point, we observe an approximately linear dispersion with vanishing spectral weight. Second, we compare two analytical frameworks that reproduce the observed features. The first is a hard-core boson approach, which includes (i) an effective staggered boson model at zero magnetic field, (ii) perturbation theory applied to the one-third magnetization plateau, and (iii) a self-consistent mean-field Schwinger boson theory (SBT). The second framework is based on a variational supersolid quantum dimer model (QDM) ansatz, combined with a single-mode approximation. The SBT captures the broad continuum, the <g:math xmlns:g="http://www.w3.org/1998/Math/MathML"> <g:mi>M</g:mi> </g:math> -point minimum, and linear dispersion at <h:math xmlns:h="http://www.w3.org/1998/Math/MathML"> <h:mi mathvariant="normal">Γ</h:mi> </h:math> , whereas the QDM reproduces the roton minimum and linear dispersion at finite momentum near <j:math xmlns:j="http://www.w3.org/1998/Math/MathML"> <j:mi mathvariant="normal">Γ</j:mi> </j:math> . Remarkably, both the QDM wave function and the DMRG ground state exhibit nearly identical structure factors with pronounced transverse photonlike excitations. Together, our comprehensive theoretical and numerical analysis elucidates the microscopic origin of supersolid excitations in the XXZ triangular-lattice model and their proximity to a spin-liquid phase observed experimentally.

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Journal
Physical review. B./Physical review. B
Published
2025-11-20
DOI
https://doi.org/10.1103/xdwz-8k94
Primary Topic
Theoretical and Computational Physics
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article
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article

Unconventional spin dynamics and supersolid excitations in the triangular-lattice XXZ model

Roderich Moessner, Frank Pollmann, R. Flores-Calderón
Physical review. B./Physical review. B
Theoretical and Computational Physics
article

Unconventional spin dynamics and supersolid excitations in the triangular-lattice XXZ model

Roderich Moessner, Frank Pollmann, R. Flores-Calderón
article en

Abstract

Motivated by recent experiments, we investigate the spin- <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:mfrac> <a:mn>1</a:mn> <a:mn>2</a:mn> </a:mfrac> </a:math> XXZ model on the triangular lattice with strong Ising anisotropy, combining large-scale numerical simulations and analytical methods to uncover unconventional spin dynamics at <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"> <b:mrow> <b:mi>T</b:mi> <b:mo>=</b:mo> <b:mn>0</b:mn> </b:mrow> </b:math> . First, we compute the dynamical spin structure factor using density matrix renormalization group (DMRG) simulations and find excellent agreement with inelastic neutron scattering data on the layered compound <c:math xmlns:c="http://www.w3.org/1998/Math/MathML"> <c:mrow> <c:msub> <c:mtext>K</c:mtext> <c:mn>2</c:mn> </c:msub> <c:mtext>Co</c:mtext> <c:msub> <c:mrow> <c:mo>(</c:mo> <c:msub> <c:mtext>SeO</c:mtext> <c:mn>3</c:mn> </c:msub> <c:mo>)</c:mo> </c:mrow> <c:mn>2</c:mn> </c:msub> </c:mrow> </c:math> . The low-energy spectrum reveals a rotonlike minimum at the <d:math xmlns:d="http://www.w3.org/1998/Math/MathML"> <d:mi>M</d:mi> </d:math> point, absent in linear spin-wave theory, accompanied by peak intensity and a broad continuum above it. Near the <e:math xmlns:e="http://www.w3.org/1998/Math/MathML"> <e:mi mathvariant="normal">Γ</e:mi> </e:math> point, we observe an approximately linear dispersion with vanishing spectral weight. Second, we compare two analytical frameworks that reproduce the observed features. The first is a hard-core boson approach, which includes (i) an effective staggered boson model at zero magnetic field, (ii) perturbation theory applied to the one-third magnetization plateau, and (iii) a self-consistent mean-field Schwinger boson theory (SBT). The second framework is based on a variational supersolid quantum dimer model (QDM) ansatz, combined with a single-mode approximation. The SBT captures the broad continuum, the <g:math xmlns:g="http://www.w3.org/1998/Math/MathML"> <g:mi>M</g:mi> </g:math> -point minimum, and linear dispersion at <h:math xmlns:h="http://www.w3.org/1998/Math/MathML"> <h:mi mathvariant="normal">Γ</h:mi> </h:math> , whereas the QDM reproduces the roton minimum and linear dispersion at finite momentum near <j:math xmlns:j="http://www.w3.org/1998/Math/MathML"> <j:mi mathvariant="normal">Γ</j:mi> </j:math> . Remarkably, both the QDM wave function and the DMRG ground state exhibit nearly identical structure factors with pronounced transverse photonlike excitations. Together, our comprehensive theoretical and numerical analysis elucidates the microscopic origin of supersolid excitations in the XXZ triangular-lattice model and their proximity to a spin-liquid phase observed experimentally.

Physical review. B./Physical review. BVol. 112(18)
Max Planck Institute for the Physics of Complex Systems (DE), Technical University of Munich (DE)
Deutsche Forschungsgemeinschaft
Openalex Percentile: Top 81%
Theoretical and Computational Physics
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