Ionization and temperature measurements in warm dense copper using x-ray absorption spectroscopy

We detail experimental results inferring ionization and temperature for warm dense copper plasmas at several times solid density (15–25 <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:msup> <a:mrow> <a:mi mathvariant="normal">g</a:mi> <a:mo>/</a:mo> <a:mi>cm</a:mi> </a:mrow> <a:mn>3</a:mn> </a:msup> </a:math> ) and temperatures of 10–21 eV. Experiments performed at the OMEGA Laser Facility generate uniform warm dense matter conditions via symmetric shock compression of a buried copper layer. The plasma is probed with a laser-generated x-ray source to collect the K-shell x-ray absorption spectrum. Fitting bound-bound absorption contributions from constituent charge states of copper provides an estimated <c:math xmlns:c="http://www.w3.org/1998/Math/MathML"> <c:mover> <c:mi>Z</c:mi> <c:mo>¯</c:mo> </c:mover> </c:math> of approximately 4–7 for these warm dense copper plasmas. We find that these partially ionized plasmas have K-edge shifts of 12–30 eV and bound-bound resonance <d:math xmlns:d="http://www.w3.org/1998/Math/MathML"> <d:mrow> <d:mn>1</d:mn> <d:mi>s</d:mi> <d:mo>→</d:mo> <d:mn>3</d:mn> <d:mi>p</d:mi> </d:mrow> </d:math> absorption shifts of 4–26 eV with respect to the cold K edge. This study provides necessary experimental data to improve ionization and opacity models in the warm dense matter regime.

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Journal
Physical Review Research
Published
2026-01-30
DOI
https://doi.org/10.1103/7vf4-flqv
Primary Topic
Electron and X-Ray Spectroscopy Techniques
Type
article
Field-Weighted Citation Impact
0.00

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article

Ionization and temperature measurements in warm dense copper using x-ray absorption spectroscopy

Richard A. London, Mike MacDonald, M. Millot, Edward V. Marley et al.
Physical Review Research
Electron and X-Ray Spectroscopy Techniques
article

Ionization and temperature measurements in warm dense copper using x-ray absorption spectroscopy

Richard A. London, Mike MacDonald, M. Millot, Edward V. Marley, H. A. Scott, T. Döppner, D. A. Chin, J. Emig, P. A. Sterne, T. Cordova, F. Coppari, F. N. Beg, Ole Hansen, Phil Nilson
article en

Abstract

We detail experimental results inferring ionization and temperature for warm dense copper plasmas at several times solid density (15–25 <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:msup> <a:mrow> <a:mi mathvariant="normal">g</a:mi> <a:mo>/</a:mo> <a:mi>cm</a:mi> </a:mrow> <a:mn>3</a:mn> </a:msup> </a:math> ) and temperatures of 10–21 eV. Experiments performed at the OMEGA Laser Facility generate uniform warm dense matter conditions via symmetric shock compression of a buried copper layer. The plasma is probed with a laser-generated x-ray source to collect the K-shell x-ray absorption spectrum. Fitting bound-bound absorption contributions from constituent charge states of copper provides an estimated <c:math xmlns:c="http://www.w3.org/1998/Math/MathML"> <c:mover> <c:mi>Z</c:mi> <c:mo>¯</c:mo> </c:mover> </c:math> of approximately 4–7 for these warm dense copper plasmas. We find that these partially ionized plasmas have K-edge shifts of 12–30 eV and bound-bound resonance <d:math xmlns:d="http://www.w3.org/1998/Math/MathML"> <d:mrow> <d:mn>1</d:mn> <d:mi>s</d:mi> <d:mo>→</d:mo> <d:mn>3</d:mn> <d:mi>p</d:mi> </d:mrow> </d:math> absorption shifts of 4–26 eV with respect to the cold K edge. This study provides necessary experimental data to improve ionization and opacity models in the warm dense matter regime.

Physical Review ResearchVol. 8(1)
Lawrence Livermore National Laboratory (US), University of California San Diego (US), Sandia National Laboratories (US), University of Rochester (US)
U.S. Department of Energy, University of Rochester, National Nuclear Security Administration, Laboratory Directed Research and Development, Lawrence Livermore National Laboratory
Openalex Percentile: Top 99%
Electron and X-Ray Spectroscopy Techniques
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