Ionization and temperature measurements in warm dense copper using x-ray absorption spectroscopy
We detail experimental results inferring ionization and temperature for warm dense copper plasmas at several times solid density (15–25 <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"> <a:msup> <a:mrow> <a:mi mathvariant="normal">g</a:mi> <a:mo>/</a:mo> <a:mi>cm</a:mi> </a:mrow> <a:mn>3</a:mn> </a:msup> </a:math> ) and temperatures of 10–21 eV. Experiments performed at the OMEGA Laser Facility generate uniform warm dense matter conditions via symmetric shock compression of a buried copper layer. The plasma is probed with a laser-generated x-ray source to collect the K-shell x-ray absorption spectrum. Fitting bound-bound absorption contributions from constituent charge states of copper provides an estimated <c:math xmlns:c="http://www.w3.org/1998/Math/MathML"> <c:mover> <c:mi>Z</c:mi> <c:mo>¯</c:mo> </c:mover> </c:math> of approximately 4–7 for these warm dense copper plasmas. We find that these partially ionized plasmas have K-edge shifts of 12–30 eV and bound-bound resonance <d:math xmlns:d="http://www.w3.org/1998/Math/MathML"> <d:mrow> <d:mn>1</d:mn> <d:mi>s</d:mi> <d:mo>→</d:mo> <d:mn>3</d:mn> <d:mi>p</d:mi> </d:mrow> </d:math> absorption shifts of 4–26 eV with respect to the cold K edge. This study provides necessary experimental data to improve ionization and opacity models in the warm dense matter regime.
Authors
- Richard A. London (ORCID: https://orcid.org/0000-0003-1853-5815)
- Mike MacDonald
- M. Millot (ORCID: https://orcid.org/0000-0003-4414-3532)
- Edward V. Marley (ORCID: https://orcid.org/0000-0001-7030-944X)
- H. A. Scott
- T. Döppner (ORCID: https://orcid.org/0000-0002-5703-7125)
- D. A. Chin (ORCID: https://orcid.org/0000-0003-0118-7690)
- J. Emig
- P. A. Sterne (ORCID: https://orcid.org/0000-0002-6398-3185)
- T. Cordova (ORCID: https://orcid.org/0000-0003-1877-7953)
- F. Coppari (ORCID: https://orcid.org/0000-0003-1592-3898)
- F. N. Beg (ORCID: https://orcid.org/0000-0003-0391-8944)
- Ole Hansen (ORCID: https://orcid.org/0000-0002-6090-8323)
- Phil Nilson
Institutions
- Lawrence Livermore National Laboratory (US)
- University of California San Diego (US)
- Sandia National Laboratories (US)
- University of Rochester (US)
Publication Details
- Journal
- Physical Review Research
- Published
- 2026-01-30
- DOI
- https://doi.org/10.1103/7vf4-flqv
- Primary Topic
- Electron and X-Ray Spectroscopy Techniques
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- U.S. Department of Energy
- University of Rochester
- National Nuclear Security Administration
- Laboratory Directed Research and Development
- Lawrence Livermore National Laboratory