Mott Insulator Polariton in a MoSe <sub>2</sub> /WS <sub>2</sub> Moiré Lattice

Transition metal dichalcogenide moiré superlattices host rich correlated electronic states with high tunability. Their integration with optical cavities offers a new platform to explore hybrid light-matter interactions. However, the interplay between electron correlations and polariton formation remains uncharted. Here, we demonstrate the realization of a Mott insulator polariton in a gate-tunable MoSe<sub>2</sub>/WS<sub>2</sub> moiré heterostructure embedded in a microcavity at the moiré lattice filling of ν = 1. A silver top layer was used to gate the moiré lattice and form the cavity reflection layer. Magnetic field studies indicate that the polaritons inherit valley Zeeman splitting from the moiré excitons, exhibiting saturation behavior similar to that of the bare moiré excitons. Our work establishes moiré polaritons as an electrically and magnetically tunable platform for engineering the quantum phases of light and matter.

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Publication Details

Journal
Nano Letters
Published
2025-10-17
DOI
https://doi.org/10.1021/acs.nanolett.5c04233
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
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article

Mott Insulator Polariton in a MoSe 2 /WS 2 Moiré Lattice

Takashi Taniguchi, Kenji Watanabe, Jie Gu, Xin Guo et al.
Nano Letters
Strong Light-Matter Interactions
article

Mott Insulator Polariton in a MoSe 2 /WS 2 Moiré Lattice

Takashi Taniguchi, Kenji Watanabe, Jie Gu, Xin Guo, Zhanghai Chen, Hao Ge
article en

Abstract

Transition metal dichalcogenide moiré superlattices host rich correlated electronic states with high tunability. Their integration with optical cavities offers a new platform to explore hybrid light-matter interactions. However, the interplay between electron correlations and polariton formation remains uncharted. Here, we demonstrate the realization of a Mott insulator polariton in a gate-tunable MoSe<sub>2</sub>/WS<sub>2</sub> moiré heterostructure embedded in a microcavity at the moiré lattice filling of ν = 1. A silver top layer was used to gate the moiré lattice and form the cavity reflection layer. Magnetic field studies indicate that the polaritons inherit valley Zeeman splitting from the moiré excitons, exhibiting saturation behavior similar to that of the bare moiré excitons. Our work establishes moiré polaritons as an electrically and magnetically tunable platform for engineering the quantum phases of light and matter.

Nano LettersVol. 25(43)
Xiamen University (CN), National Institute for Materials Science (JP), Fudan University (CN), Physical Sciences (United States) (US), Science and Technology on Surface Physics and Chemistry Laboratory (CN), State Key Laboratory of Surface Physics, Xiamen University of Technology (CN)
Openalex Percentile: Top 76%
Strong Light-Matter Interactions
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Mott Insulator Polariton in a MoSe <sub>2</sub> /WS <sub>2</sub> Moiré Lattice — Takashi Taniguchi, Kenji Watanabe, et al. · Nano Letters (2025) | TGRS Research Map | TGRS