Distributed direct air capture by carbon nanofiber air filters
The rising atmospheric CO<sub>2</sub> concentration is one of the biggest challenges human civilization faces. Direct air capture (DAC) that removes CO<sub>2</sub> from the atmosphere provides great potential in carbon neutralization. However, the massive land use and capital investment of centralized DAC plants and the energy-intensive process of adsorbent regeneration limit its wide employment. We develop a distributed carbon nanofiber (CNF)-based DAC air filter capable of adsorbing CO<sub>2</sub> downstream in ventilation systems. The DAC air filter not only has the potential to remove 596 MtCO<sub>2</sub> year<sup>-1</sup> globally but can also decrease energy consumption in existing building systems. The CNF-based adsorbent has a capacity of 4 mmol/g and can be regenerated via solar thermal or electrothermal methods with low carbon footprints. Through life cycle assessment, the CNF air filter shows a carbon removal efficiency of 92.1% from cradle to grave. Additionally, techno-economic analysis estimates a cost of $209 to 668 in capturing and storing 1 tonne of CO<sub>2</sub> from direct air.
Authors
- Gangbin Yan (ORCID: https://orcid.org/0000-0002-4711-9063)
- Amar Ruthen (ORCID: https://orcid.org/0000-0002-9485-057X)
- Hernan E. Delgado (ORCID: https://orcid.org/0000-0001-8969-6523)
- Adarsh Suresh (ORCID: https://orcid.org/0000-0001-5981-9932)
- David B. Mitzi (ORCID: https://orcid.org/0000-0001-5189-4612)
- Po‐Chun Hsu (ORCID: https://orcid.org/0000-0002-6509-9377)
- Yuanke Chen (ORCID: https://orcid.org/0009-0007-0148-1378)
- Genesis Higueros (ORCID: https://orcid.org/0009-0005-6653-1693)
- Amgad Elgowainy (ORCID: https://orcid.org/0000-0003-3713-4654)
- Yu Han (ORCID: https://orcid.org/0000-0001-7905-0032)
- Chenxi Sui (ORCID: https://orcid.org/0000-0003-2244-8431)
- Ronghui Wu (ORCID: https://orcid.org/0000-0002-0752-9383)
- Qingsong Fan (ORCID: https://orcid.org/0000-0001-8555-769X)
- Qizhang Li (ORCID: https://orcid.org/0000-0002-5454-4578)
- Edward Luo (ORCID: https://orcid.org/0009-0009-5822-4473)
- Chong Liu (ORCID: https://orcid.org/0000-0003-4851-7888)
- Yi Xie (ORCID: https://orcid.org/0000-0003-0310-107X)
Institutions
- Argonne National Laboratory (US)
- Duke University (US)
- Nanyang Technological University (SG)
- University of Chicago (US)
Publication Details
- Journal
- Science Advances
- Published
- 2025-10-17
- DOI
- https://doi.org/10.1126/sciadv.adv6846
- Citations
- 2
- Primary Topic
- Carbon Dioxide Capture Technologies
- Type
- article
- Field-Weighted Citation Impact
- 1.43