Multiscale stress dynamics in sheared liquid foams revealed by tomo-rheoscopy
Rheology aims at quantifying the response of materials to mechanical forcing. However, standard rheometers provide only global macroscopic quantities, such as viscoelastic moduli. They fail to capture the heterogeneous flow of soft amorphous materials at the mesoscopic scale, arising from the rearrangements of the microstructural elements, that must be accounted for to build predictive models. To address this experimental challenge, we have combined shear rheometry and time-resolved X-ray micro-tomography on 3D liquid foams used as model soft jammed materials, yielding a unique access to the stresses and contact network topology at the bubble scale. We reveal a universal scaling behavior of the local stress build-up and relaxation associated with topological modifications. Moreover, these plastic events redistribute stress non-locally, as if the foam were an elastic medium subjected to a quadrupolar deformation. Our findings clarify how the macroscopic elastoplastic behavior of amorphous materials emerges from the spatiotemporal stress variations induced by microstructural rearrangements.
Authors
- Stefan J. Gstöhl (ORCID: https://orcid.org/0000-0003-1842-3573)
- Christian M. Schlepütz (ORCID: https://orcid.org/0000-0002-0485-2708)
- Cyrille Claudet (ORCID: https://orcid.org/0000-0002-7733-8283)
- Rajmund Mokso (ORCID: https://orcid.org/0000-0002-2245-2775)
- Christophe Raufaste (ORCID: https://orcid.org/0000-0003-4328-7438)
- Benjamin Dollet (ORCID: https://orcid.org/0000-0002-1756-7543)
- Stéphane Santucci (ORCID: https://orcid.org/0000-0002-6323-191X)
- Florian Schott (ORCID: https://orcid.org/0000-0003-3467-3820)
Institutions
- École Normale Supérieure de Lyon (FR)
- Centre National de la Recherche Scientifique (FR)
- Institut Universitaire de France (FR)
- Lund University (SE)
- Université Côte d'Azur (FR)
- Paul Scherrer Institute (CH)
- Laboratoire de Physique de l'ENS de Lyon (FR)
- Laboratoire Interdisciplinaire de Physique (FR)
- Immune Therapy Holdings (Sweden) (SE)
- Institut de Physique de Nice (FR)
- Unité de Mathématiques Pures et Appliquées (FR)
- Swiss Light Source
- Université Grenoble Alpes (FR)
- Technical University of Denmark (DK)
Publication Details
- Journal
- Nature Communications
- Published
- 2025-10-16
- DOI
- https://doi.org/10.1038/s41467-025-64412-z
- Citations
- 3
- Primary Topic
- Pickering emulsions and particle stabilization
- Type
- article
- Field-Weighted Citation Impact
- 1.55
Funders
- National Science Foundation
- Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung
- Lunds Universitet
- Paul Scherrer Institut
- Vetenskapsrådet
- Centre National de la Recherche Scientifique
- École Normale Supérieure de Lyon