Coffee Drying as a Catalytic Gas–Solid Dehydration Analogy: A Desiccant-Assisted Theoretical Framework

Coffee drying in humid regions is frequently hindered by high rainfall and elevated relative humidity during peak harvest, prolonging drying times and risking microbial spoilage and quality deterioration. This study introduces a novel framework in which low-temperature drying is reframed as a gas–solid dehydration reaction, promoted by a catalyst analog represented by regenerable desiccants integrated into the inlet air stream to lower the humidity ratio (ΔY) and intensify the evaporation driving force. Two adsorbents, silica gel type A and zeolite 13X, were evaluated using a coupled reactor model linking fixed-bed adsorption kinetics with tensorial heat–mass transport in a 70 kg batch of parchment coffee arranged in a 0.20 m thick bed. Drying simulations from 53% to 12% (wb) at 40, 45, and 50 °C showed time reductions of 35–37% with silica gel and 44–57% with zeolite, yielding kinetic promotion factors of up to 2.3× relative to the control. Breakthrough analysis supported a dual-bed alternation strategy, with regeneration at ≤130 °C for silica and moderately higher for zeolite. A nomograph was developed to scale desiccant requirements across airflow and ΔY targets. These results confirm the feasibility and scalability of desiccant-assisted drying, providing a modular intensification pathway for farm-scale coffee processing.