Identifying Electronic Doorway States in Secondary Electron Emission from Layered Materials

We investigate the secondary low-energy electron emission induced by inelastic electron scattering from graphene and layered materials thereof. By applying a coincidence detection of the primary scattered and the emitted secondary electron we unravel pronounced resonance features otherwise overshadowed by the largely structureless secondary electron energy distribution. Supported by density functional theory calculations we show that these structures are the signature of prominent resonances above the vacuum threshold which originate from interlayer states acting as a doorway state for electron emission. Remarkably, some of these doorway states open up only for samples with more than five layers.

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Publication Details

Journal
Physical Review Letters
Published
2025-10-15
DOI
https://doi.org/10.1103/qls7-tr4v
Primary Topic
Electron and X-Ray Spectroscopy Techniques
Type
article
Field-Weighted Citation Impact
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article

Identifying Electronic Doorway States in Secondary Electron Emission from Layered Materials

Joachim Burgdörfer, Florian Libisch, Alessandra Bellissimo, Dieter Hofmann et al.
Physical Review Letters
Electron and X-Ray Spectroscopy Techniques
article

Identifying Electronic Doorway States in Secondary Electron Emission from Layered Materials

Joachim Burgdörfer, Florian Libisch, Alessandra Bellissimo, Dieter Hofmann, Wolfgang Werner, Péter Richter, Thomas Seyller, Anna Niggas, R. Wilhelm, Florian Simperl, Johannes Kero, Felix Blödorn, Maosheng Hao, Melvin Cap
article en

Abstract

We investigate the secondary low-energy electron emission induced by inelastic electron scattering from graphene and layered materials thereof. By applying a coincidence detection of the primary scattered and the emitted secondary electron we unravel pronounced resonance features otherwise overshadowed by the largely structureless secondary electron energy distribution. Supported by density functional theory calculations we show that these structures are the signature of prominent resonances above the vacuum threshold which originate from interlayer states acting as a doorway state for electron emission. Remarkably, some of these doorway states open up only for samples with more than five layers.

Physical Review LettersVol. 135(16)
TU Wien (AT), Chemnitz University of Technology (DE)
Openalex Percentile: Top 72%
Electron and X-Ray Spectroscopy Techniques
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Identifying Electronic Doorway States in Secondary Electron Emission from Layered Materials — Joachim Burgdörfer, Florian Libisch, et al. · Physical Review Letters (2025) | TGRS Research Map | TGRS