Cascaded exciton-photon coupling in hybrid Tamm plasmon–Fabry-Pérot cavities embedded with perovskite quantum dots

We demonstrate a hybrid photonic architecture in which excitons from CsPbBr<sub>3</sub> quantum dots (QDs) strongly couple with both Tamm plasmon (TP) and Fabry-Pérot (FP) resonances, leading to the formation of hybridized exciton-polariton states. The QDs exhibit a binding energy of ∼61.5 <i>meV</i>, ensuring stable exciton states at room temperature. Reflectance spectrum reveals clear mode anti-crossings and large Rabi splittings exceeding 220 <i>meV</i>, unambiguously confirming strong light-matter coupling. By systematically tuning the cavity spacer thicknesses, the evolution of hybrid upper and lower polariton branches is experimentally mapped and quantitatively described by a coupled-oscillator model. Momentum-resolved spectroscopy further verifies a cascaded coupling process, wherein QD excitons first hybridize with the TP mode and subsequently with the FP mode. The resulting polaritonic states exhibit spectral narrowing, asymmetric emission, and accelerated radiative decay. These findings provide experimental evidence of exciton-polaritons in a TP-FP dual-cavity system and establish a compact, silicon-compatible platform for multifunctional photonic and photoelectronic applications.

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Publication Details

Journal
Optics Express
Published
2025-10-15
DOI
https://doi.org/10.1364/oe.576663
Primary Topic
Photonic and Optical Devices
Type
article
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article

Cascaded exciton-photon coupling in hybrid Tamm plasmon–Fabry-Pérot cavities embedded with perovskite quantum dots

Chia‐Jung Lee, Wen-Chi Huang, Y. D. Yao, Hsu‐Cheng Hsu et al.
Optics Express
Photonic and Optical Devices
article

Cascaded exciton-photon coupling in hybrid Tamm plasmon–Fabry-Pérot cavities embedded with perovskite quantum dots

Chia‐Jung Lee, Wen-Chi Huang, Y. D. Yao, Hsu‐Cheng Hsu, Ya‐Ju Lee, Gong‐Ru Lin, Yu‐Wen Huang, Chunyan Su, S.Y. Wu, May Yen
article en

Abstract

We demonstrate a hybrid photonic architecture in which excitons from CsPbBr<sub>3</sub> quantum dots (QDs) strongly couple with both Tamm plasmon (TP) and Fabry-Pérot (FP) resonances, leading to the formation of hybridized exciton-polariton states. The QDs exhibit a binding energy of ∼61.5 <i>meV</i>, ensuring stable exciton states at room temperature. Reflectance spectrum reveals clear mode anti-crossings and large Rabi splittings exceeding 220 <i>meV</i>, unambiguously confirming strong light-matter coupling. By systematically tuning the cavity spacer thicknesses, the evolution of hybrid upper and lower polariton branches is experimentally mapped and quantitatively described by a coupled-oscillator model. Momentum-resolved spectroscopy further verifies a cascaded coupling process, wherein QD excitons first hybridize with the TP mode and subsequently with the FP mode. The resulting polaritonic states exhibit spectral narrowing, asymmetric emission, and accelerated radiative decay. These findings provide experimental evidence of exciton-polaritons in a TP-FP dual-cavity system and establish a compact, silicon-compatible platform for multifunctional photonic and photoelectronic applications.

Optics ExpressVol. 33(22)
National Sun Yat-sen University (TW), National Taiwan University (TW)
Openalex Percentile: Top 71%
Photonic and Optical Devices
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