Optical interference effect in strong-field electronic coherence spectroscopy

The authors present a combined experimental and theoretical study of strong-field-induced electronic coherences in argon and molecular nitrogen ions as a step towards strong-field coherent control in molecular chemistry. They find that nonsequential double ionization in the low-intensity region of the focal volume can reduce the visibility of coherence generated by two-pulse sequential ionization, and quantify the importance of pulse shape and spectral characteristics for isolating the desired coherence signals.

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Publication Details

Journal
Physical review. A/Physical review, A
Published
2025-10-14
DOI
https://doi.org/10.1103/rkdq-5skq
Primary Topic
Laser-Matter Interactions and Applications
Type
article
Field-Weighted Citation Impact
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Optical interference effect in strong-field electronic coherence spectroscopy

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Optical interference effect in strong-field electronic coherence spectroscopy

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article en

Abstract

The authors present a combined experimental and theoretical study of strong-field-induced electronic coherences in argon and molecular nitrogen ions as a step towards strong-field coherent control in molecular chemistry. They find that nonsequential double ionization in the low-intensity region of the focal volume can reduce the visibility of coherence generated by two-pulse sequential ionization, and quantify the importance of pulse shape and spectral characteristics for isolating the desired coherence signals.

Physical review. A/Physical review, AVol. 112(4)
Kennesaw State University (US), Kansas State University (US), SLAC National Accelerator Laboratory (US), Stanford University (US)
Openalex Percentile: Top 77%
Laser-Matter Interactions and Applications
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