Encoding quadrupolar capillary information into saddle-shaped objects for self-assembly

Capillary-driven self-assembly at liquid interfaces, often illustrated by the ``Cheerios effect,'' has been limited to simple configurations. By introducing anisotropic, saddle-shaped particles, we demonstrate how quadrupolar capillary interactions can be encoded to achieve both end-to-end and side-by-side attraction; what we call the ``Pringles effect.'' Our theoretical model and experiments with 3D-printed objects reveal a versatile route to reprogrammable mesoscale assemblies, bridging capillarity and design for complex self-organization.

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Publication Details

Journal
Physical Review Fluids
Published
2025-10-14
DOI
https://doi.org/10.1103/f3tr-kby1
Primary Topic
Supramolecular Self-Assembly in Materials
Type
article
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article

Encoding quadrupolar capillary information into saddle-shaped objects for self-assembly

Nicolas Vandewalle, Megan Delens
Physical Review Fluids
Supramolecular Self-Assembly in Materials
article

Encoding quadrupolar capillary information into saddle-shaped objects for self-assembly

Nicolas Vandewalle, Megan Delens
article en

Abstract

Capillary-driven self-assembly at liquid interfaces, often illustrated by the ``Cheerios effect,'' has been limited to simple configurations. By introducing anisotropic, saddle-shaped particles, we demonstrate how quadrupolar capillary interactions can be encoded to achieve both end-to-end and side-by-side attraction; what we call the ``Pringles effect.'' Our theoretical model and experiments with 3D-printed objects reveal a versatile route to reprogrammable mesoscale assemblies, bridging capillarity and design for complex self-organization.

Physical Review FluidsVol. 10(10)
University of Liège (BE)
Openalex Percentile: Top 81%
Supramolecular Self-Assembly in Materials
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