High-magnetic-field phases in U <sub>1-x</sub> Th <sub>x</sub> Te <sub>2</sub>

At temperatures <i>T</i> much lower than its superconducting critical temperature <i>T</i><sub>c</sub> = 2.1 K, the heavy fermion superconductor UTe<sub>2</sub> has a unique phase diagram of magnetic field <i>H</i> vs. φ and θ, angles <i>H</i> is tilted from the <i>b</i>-axis toward the <i>a</i>- and <i>c</i>-axes, respectively, of its orthorhombic unit cell. The phase diagram contains three distinct superconducting phases: SC<sub>1</sub> in which φ and θ extend from 0 to 90° and <i>H</i> ≤ ~15 T; SC<sub>2</sub> for φ ≤ ~7°, θ ≤ ~4° and ~15 T ≤ <i>H</i> ≤ <i>H</i><sub>m</sub> = ~35 T, the onset of the magnetic field polarized (FP) phase, and SC<sub>FP</sub> which resides entirely within the FP phase in a pocket of superconductivity extending from θ ≈ 20° to 40° and from ~40 T to above 60 T. We studied the evolution of the <i>H</i> vs. θ phase diagram for Th concentrations 0.005 ≤ <i>x</i> ≤ 0.047 in the U<sub>1-x</sub>Th<sub>x</sub>Te<sub>2</sub> system at ~0.6 K. Within this range of <i>x</i> values, SC<sub>1</sub> extends over 0 ≤ θ ≤ 90° and <i>H</i> ≤ ~10 T for <i>x</i> = 0.047, while SC<sub>2</sub> is suppressed. The SC<sub>FP</sub> and FP phases are unaffected to <i>x</i> = 0.02 but are completely suppressed in the region <i>x</i> = 0.025 to 0.047 where the residual resistance ratio <i>RRR</i> ~3 indicates a significant amount of disorder. These results complement recent studies of nonsuperconducting disordered UTe<sub>2</sub> single crystals in which the SC<sub>1</sub> and SC<sub>2</sub> phases are absent, but the FP and so-called "orphan" SC<sub>FP</sub> phases are retained.

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Journal
Proceedings of the National Academy of Sciences
Published
2025-10-13
DOI
https://doi.org/10.1073/pnas.2521261122
Citations
1
Primary Topic
Rare-earth and actinide compounds
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article
Field-Weighted Citation Impact
1.26
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article

High-magnetic-field phases in U 1-x Th x Te 2

John Singleton, Ryan Baumbach, Joanna Bławat, Camilla M. Moir et al.
1 citations
Proceedings of the National Academy of Sciences
Rare-earth and actinide compounds
1.26
article

High-magnetic-field phases in U 1-x Th x Te 2

John Singleton, Ryan Baumbach, Joanna Bławat, Camilla M. Moir, Keke Feng, Yuhang Deng, M. Brian Maple, Eric Lee-Wong, Tyler Wannamaker
article en
1 citations

Abstract

At temperatures <i>T</i> much lower than its superconducting critical temperature <i>T</i><sub>c</sub> = 2.1 K, the heavy fermion superconductor UTe<sub>2</sub> has a unique phase diagram of magnetic field <i>H</i> vs. φ and θ, angles <i>H</i> is tilted from the <i>b</i>-axis toward the <i>a</i>- and <i>c</i>-axes, respectively, of its orthorhombic unit cell. The phase diagram contains three distinct superconducting phases: SC<sub>1</sub> in which φ and θ extend from 0 to 90° and <i>H</i> ≤ ~15 T; SC<sub>2</sub> for φ ≤ ~7°, θ ≤ ~4° and ~15 T ≤ <i>H</i> ≤ <i>H</i><sub>m</sub> = ~35 T, the onset of the magnetic field polarized (FP) phase, and SC<sub>FP</sub> which resides entirely within the FP phase in a pocket of superconductivity extending from θ ≈ 20° to 40° and from ~40 T to above 60 T. We studied the evolution of the <i>H</i> vs. θ phase diagram for Th concentrations 0.005 ≤ <i>x</i> ≤ 0.047 in the U<sub>1-x</sub>Th<sub>x</sub>Te<sub>2</sub> system at ~0.6 K. Within this range of <i>x</i> values, SC<sub>1</sub> extends over 0 ≤ θ ≤ 90° and <i>H</i> ≤ ~10 T for <i>x</i> = 0.047, while SC<sub>2</sub> is suppressed. The SC<sub>FP</sub> and FP phases are unaffected to <i>x</i> = 0.02 but are completely suppressed in the region <i>x</i> = 0.025 to 0.047 where the residual resistance ratio <i>RRR</i> ~3 indicates a significant amount of disorder. These results complement recent studies of nonsuperconducting disordered UTe<sub>2</sub> single crystals in which the SC<sub>1</sub> and SC<sub>2</sub> phases are absent, but the FP and so-called "orphan" SC<sub>FP</sub> phases are retained.

Proceedings of the National Academy of SciencesVol. 122(42)
Florida State University (US), Los Alamos National Laboratory (US), University of California San Diego (US), National High Magnetic Field Laboratory (US)
Openalex Percentile: Top 17%
Rare-earth and actinide compounds
1.26
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