Polariton Lasing at Topological States in Organic Semiconductor Lattices

Topological photonics offers a versatile platform for designing advanced photonic materials and devices, such as one-way waveguides, on-chip optical isolators, and topologically protected lasers. Recently, particular interest has emerged in exploring topologically protected polariton lasing. However, current topological polariton lasers mainly rely on inorganic semiconductors, suffering from cryogenic temperature operation and limited applicability due to the small binding energies of Wannier-Mott excitons. Here, we realize room-temperature topological polariton lasers by exploiting tightly bound Frenkel excitons in organic semiconductor lattices. The Frenkel excitons strongly couple with microcavity photons to generate stable exciton polaritons. By modulation of the intra- and intercell coupling strengths of organic semiconductor lattices, room-temperature polariton lasing is achieved at topological edge states. The topological polariton laser exhibits a temperature-controlled wavelength-tunable laser output. This work demonstrates organic semiconductors as promising material systems for topological polariton devices.

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Publication Details

Journal
Nano Letters
Published
2025-10-13
DOI
https://doi.org/10.1021/acs.nanolett.5c04164
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
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article

Polariton Lasing at Topological States in Organic Semiconductor Lattices

Jiannian Yao, Libo Ma, Haiyun Dong, Min Tang et al.
Nano Letters
Strong Light-Matter Interactions
article

Polariton Lasing at Topological States in Organic Semiconductor Lattices

Jiannian Yao, Libo Ma, Haiyun Dong, Min Tang, Qin Peng, Yana Vaynzof, Wu Zhou, Yong Sheng Zhao
article en

Abstract

Topological photonics offers a versatile platform for designing advanced photonic materials and devices, such as one-way waveguides, on-chip optical isolators, and topologically protected lasers. Recently, particular interest has emerged in exploring topologically protected polariton lasing. However, current topological polariton lasers mainly rely on inorganic semiconductors, suffering from cryogenic temperature operation and limited applicability due to the small binding energies of Wannier-Mott excitons. Here, we realize room-temperature topological polariton lasers by exploiting tightly bound Frenkel excitons in organic semiconductor lattices. The Frenkel excitons strongly couple with microcavity photons to generate stable exciton polaritons. By modulation of the intra- and intercell coupling strengths of organic semiconductor lattices, room-temperature polariton lasing is achieved at topological edge states. The topological polariton laser exhibits a temperature-controlled wavelength-tunable laser output. This work demonstrates organic semiconductors as promising material systems for topological polariton devices.

Nano LettersVol. 25(42)
Chinese Academy of Sciences (CN), Leibniz Institute for Solid State and Materials Research (DE), Baddi University of Emerging Sciences and Technologies (IN), Institute of Chemistry (CN), University of Chinese Academy of Sciences (CN), Technische Universität Dresden (DE)
Openalex Percentile: Top 77%
Strong Light-Matter Interactions
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Polariton Lasing at Topological States in Organic Semiconductor Lattices — Jiannian Yao, Libo Ma, et al. · Nano Letters (2025) | TGRS Research Map | TGRS