Plasmonic detection of Rashba spin-orbit coupling in monolayer transition metal dichalcogenides

Rashba spin-orbit coupling (RSOC) induces strong momentum-dependent spin splitting and plays a crucial role in fields such as spintronics and topological photonics. We here theoretically investigate the collective excitations in monolayer transition-metal dichalcogenides (ML-TMDs) hosting RSOC, and conceive an approach to precisely quantify the strength of RSOC using plasmons. We determine the electron energy loss function (EELF) and plasmon dispersions for $n$-type ML-TMDs from the dynamic dielectric function in the framework of the standard random phase approximation. In this system, both optical and acoustic plasmon modes are observed in the EELF and plasmon dispersions. Moreover, the plasmonic and spectral properties are tunable by electron density and dependent on RSOC. Crucially, we identify a minimum energy gap between the two plasmon modes to serve as a direct spectral signature of the RSOC strength. These results establish plasmons as a noninvasive, precise, and broadly tunable technique for determining RSOC in TMD van der Waals heterostructures and devices.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-10-10
DOI
https://doi.org/10.1103/pxkx-rvkl
Citations
1
Primary Topic
2D Materials and Applications
Type
article
Field-Weighted Citation Impact
0.52

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article

Plasmonic detection of Rashba spin-orbit coupling in monolayer transition metal dichalcogenides

Wen Xu, M. V. Miloševıć, Q. N. Li, Z. H. Tao et al.
1 citations
Physical review. B./Physical review. B
2D Materials and Applications
0.52
article

Plasmonic detection of Rashba spin-orbit coupling in monolayer transition metal dichalcogenides

Wen Xu, M. V. Miloševıć, Q. N. Li, Z. H. Tao, Yu-He Li, Yiming Xiao, D. Neilson, François Maria Peeters
article en
1 citations

Abstract

Rashba spin-orbit coupling (RSOC) induces strong momentum-dependent spin splitting and plays a crucial role in fields such as spintronics and topological photonics. We here theoretically investigate the collective excitations in monolayer transition-metal dichalcogenides (ML-TMDs) hosting RSOC, and conceive an approach to precisely quantify the strength of RSOC using plasmons. We determine the electron energy loss function (EELF) and plasmon dispersions for $n$-type ML-TMDs from the dynamic dielectric function in the framework of the standard random phase approximation. In this system, both optical and acoustic plasmon modes are observed in the EELF and plasmon dispersions. Moreover, the plasmonic and spectral properties are tunable by electron density and dependent on RSOC. Crucially, we identify a minimum energy gap between the two plasmon modes to serve as a direct spectral signature of the RSOC strength. These results establish plasmons as a noninvasive, precise, and broadly tunable technique for determining RSOC in TMD van der Waals heterostructures and devices.

Physical review. B./Physical review. BVol. 112(16)
University of Antwerp (BE), Yunnan University (CN), Chinese Academy of Sciences (CN), Universidade Federal do Ceará (BR), Institute of Solid State Physics (CN)
National Natural Science Foundation of China, Fonds Wetenschappelijk Onderzoek, China Scholarship Council, Vlaamse regering
Openalex Percentile: Top 32%
2D Materials and Applications
0.52
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