Conv-TssNet: A time-domain signal separation network based on cepstral analysis for direct absorption spectroscopy with interference features

This work presents Conv-TssNet, a fully convolutional neural network that integrates cepstral analysis for end-to-end separation of overlapping absorption signals directly in the optical time domain. Trained on a large-scale HITRAN-based dataset augmented with realistic baseline perturbations and spectroscopic variability, Conv-TssNet demonstrates robust generalization across diverse gas mixtures and measurement conditions, achieving high-fidelity reconstruction with mean scale-invariant signal-to-noise ratio (SI-SNR) values of 37.2 dB and 40.5 dB for target and background components, respectively. Experimental validation in a premixed CH 4 /air flat-flame burner confirms accurate and repeatable retrievals of temperature and CO concentration, with uncertainties as low as 14 K and 0.14%, respectively. Compared to the interference-feature baseline transform and background subtraction (IFBTBS) method, Conv-TssNet significantly reduces retrieval uncertainties and demonstrates superior noise immunity under turbulence-induced distortions. It maintains temperature deviations below 3.33% with 2.30% uncertainty at a high distortion level ( c 1 / 2 = 3 . 0 ), compared to 7.25% deviation and 5.10% uncertainty with IFBTBS, and accelerates computational speed by approximately 900-fold, enabling real-time, in situ applications. This study represents the first cross-domain adaptation of deep time-domain speech separation architectures to laser absorption spectroscopy, establishing a novel framework for applying deep learning to complex optical diagnostics. Future work will focus on extending the proposed network to multi-species spectral separation, developing integrated retrieval-inference frameworks, and incorporating uncertainty-aware modeling to enhance robustness for practical field deployments. • A fully convolutional neural network, Conv-TssNet, that integrates cepstral analysis for end-to-end separation of overlapping absorption signals in the optical time domain, is proposed. • Trained on a large-scale HITRAN-based dataset with baseline perturbations and spectroscopic variability, Conv-TssNet achieves high-fidelity reconstruction (SI-SNR up to 40.5 dB). • Experimental validation in CH 4 /air flat-flame burner confirms accurate retrievals of temperature (±18 K) and CO concentration (±0.18 %). • Compared with IFBTBS, Conv-TssNet reduces retrieval uncertainties, improves noise robustness under turbulence (3.33 % vs 7.25 % deviation), and accelerates computation 900×.

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Publication Details

Journal
Applications in Energy and Combustion Science
Published
2025-10-10
DOI
https://doi.org/10.1016/j.jaecs.2025.100409
Primary Topic
Spectroscopy and Laser Applications
Type
article
Field-Weighted Citation Impact
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article

Conv-TssNet: A time-domain signal separation network based on cepstral analysis for direct absorption spectroscopy with interference features

Xing Chao, Zihao Song, Aamir Farooq, Xiaoliang Chen et al.
Applications in Energy and Combustion Science
Spectroscopy and Laser Applications
article

Conv-TssNet: A time-domain signal separation network based on cepstral analysis for direct absorption spectroscopy with interference features

Xing Chao, Zihao Song, Aamir Farooq, Xiaoliang Chen, Zhenhai Wang, Weitian Wang, Pengfei Fu
article en

Abstract

This work presents Conv-TssNet, a fully convolutional neural network that integrates cepstral analysis for end-to-end separation of overlapping absorption signals directly in the optical time domain. Trained on a large-scale HITRAN-based dataset augmented with realistic baseline perturbations and spectroscopic variability, Conv-TssNet demonstrates robust generalization across diverse gas mixtures and measurement conditions, achieving high-fidelity reconstruction with mean scale-invariant signal-to-noise ratio (SI-SNR) values of 37.2 dB and 40.5 dB for target and background components, respectively. Experimental validation in a premixed CH 4 /air flat-flame burner confirms accurate and repeatable retrievals of temperature and CO concentration, with uncertainties as low as 14 K and 0.14%, respectively. Compared to the interference-feature baseline transform and background subtraction (IFBTBS) method, Conv-TssNet significantly reduces retrieval uncertainties and demonstrates superior noise immunity under turbulence-induced distortions. It maintains temperature deviations below 3.33% with 2.30% uncertainty at a high distortion level ( c 1 / 2 = 3 . 0 ), compared to 7.25% deviation and 5.10% uncertainty with IFBTBS, and accelerates computational speed by approximately 900-fold, enabling real-time, in situ applications. This study represents the first cross-domain adaptation of deep time-domain speech separation architectures to laser absorption spectroscopy, establishing a novel framework for applying deep learning to complex optical diagnostics. Future work will focus on extending the proposed network to multi-species spectral separation, developing integrated retrieval-inference frameworks, and incorporating uncertainty-aware modeling to enhance robustness for practical field deployments. • A fully convolutional neural network, Conv-TssNet, that integrates cepstral analysis for end-to-end separation of overlapping absorption signals in the optical time domain, is proposed. • Trained on a large-scale HITRAN-based dataset with baseline perturbations and spectroscopic variability, Conv-TssNet achieves high-fidelity reconstruction (SI-SNR up to 40.5 dB). • Experimental validation in CH 4 /air flat-flame burner confirms accurate retrievals of temperature (±18 K) and CO concentration (±0.18 %). • Compared with IFBTBS, Conv-TssNet reduces retrieval uncertainties, improves noise robustness under turbulence (3.33 % vs 7.25 % deviation), and accelerates computation 900×.

Applications in Energy and Combustion ScienceVol. 24
King Abdullah University of Science and Technology (SA), Zhejiang University (CN), Tsinghua University (CN)
Openalex Percentile: Top 73%
Spectroscopy and Laser Applications
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