Towards dislocation-driven quantum interconnects

A central problem in the deployment of quantum technologies is the realization of robust architectures for quantum interconnects. We propose to engineer interconnects in semiconductors and insulators by patterning spin qubits at dislocations, thus forming quasi one-dimensional lines of entangled point defects. To gain insight into the feasibility and control of dislocation-driven interconnects, we investigate the optical cycle and coherence properties of nitrogen-vacancy (NV) centers in diamond, in proximity of dislocations, using a combination of advanced first-principles calculations. We show that one can engineer spin defects with properties similar to those of their bulk counterparts, including charge stability and a favorable optical cycle, and that NV centers close to dislocations have much improved coherence properties. Finally, we predict optically detected magnetic resonance spectra that may facilitate the experimental identification of specific defect configurations. Our results provide a theoretical foundation for the engineering of one-dimensional arrays of spin defects in the solid state.

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Publication Details

Journal
npj Computational Materials
Published
2026-01-09
DOI
https://doi.org/10.1038/s41524-025-01945-3
Citations
1
Primary Topic
Semiconductor materials and devices
Type
article
Field-Weighted Citation Impact
0.00

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Towards dislocation-driven quantum interconnects

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Abstract

A central problem in the deployment of quantum technologies is the realization of robust architectures for quantum interconnects. We propose to engineer interconnects in semiconductors and insulators by patterning spin qubits at dislocations, thus forming quasi one-dimensional lines of entangled point defects. To gain insight into the feasibility and control of dislocation-driven interconnects, we investigate the optical cycle and coherence properties of nitrogen-vacancy (NV) centers in diamond, in proximity of dislocations, using a combination of advanced first-principles calculations. We show that one can engineer spin defects with properties similar to those of their bulk counterparts, including charge stability and a favorable optical cycle, and that NV centers close to dislocations have much improved coherence properties. Finally, we predict optically detected magnetic resonance spectra that may facilitate the experimental identification of specific defect configurations. Our results provide a theoretical foundation for the engineering of one-dimensional arrays of spin defects in the solid state.

npj Computational MaterialsVol. 12(1)
Argonne National Laboratory (US), University of Chicago (US), The Ohio State University (US)
U.S. Department of Energy, National Energy Research Scientific Computing Center, Midwest Integrated Center for Computational Materials, Office of Science, Basic Energy Sciences, Air Force Office of Scientific Research, Argonne National Laboratory
Openalex Percentile: Top 100%
Semiconductor materials and devices
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Towards dislocation-driven quantum interconnects — Cunzhi Zhang, Maryam Ghazisaeidi, et al. · npj Computational Materials (2026) | TGRS Research Map | TGRS