Phase transitions induced by resonant light: A phenomenological approach

We present a phenomenological framework to describe a subclass of light-induced phase transitions (LIPTs) in condensed matter systems, specifically those mediated by the resonant generation of excitons. Our approach extends the classical Landau theory by introducing dynamic coupling between the system's order parameter and complex excitonic fields, along with Langevin-type forces that drive the system toward states of minimal free energy. The model is applied in the context of all-optical resonant magnetization switching in two-dimensional magnetic materials, particularly reproducing the experimental findings for reverse magnetization by all-optical means for a monolayer CrI3. Our phenomenological model can be applied to other systems characterized by an order parameter and excitonic fields created through resonant light, offering versatility and potential to guide future experimental and theoretical studies in LIPT phenomena.

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Publication Details

Journal
The Journal of Chemical Physics
Published
2025-10-08
DOI
https://doi.org/10.1063/5.0284300
Primary Topic
Perovskite Materials and Applications
Type
article
Field-Weighted Citation Impact
0.00

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article

Phase transitions induced by resonant light: A phenomenological approach

Helgi Sigurðsson, A. Kudlis, L. S. Ricco, I. A. Shelykh
The Journal of Chemical Physics
Perovskite Materials and Applications
article

Phase transitions induced by resonant light: A phenomenological approach

Helgi Sigurðsson, A. Kudlis, L. S. Ricco, I. A. Shelykh
article en

Abstract

We present a phenomenological framework to describe a subclass of light-induced phase transitions (LIPTs) in condensed matter systems, specifically those mediated by the resonant generation of excitons. Our approach extends the classical Landau theory by introducing dynamic coupling between the system's order parameter and complex excitonic fields, along with Langevin-type forces that drive the system toward states of minimal free energy. The model is applied in the context of all-optical resonant magnetization switching in two-dimensional magnetic materials, particularly reproducing the experimental findings for reverse magnetization by all-optical means for a monolayer CrI3. Our phenomenological model can be applied to other systems characterized by an order parameter and excitonic fields created through resonant light, offering versatility and potential to guide future experimental and theoretical studies in LIPT phenomena.

The Journal of Chemical PhysicsVol. 163(14)
University of Iceland (IS), University of Warsaw (PL)
European Commission, Rannís
Openalex Percentile: Top 72%
Perovskite Materials and Applications
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