Drop Friction on Textured Lubricant-Coated Surfaces

Understanding drop friction on textured surfaces has implications in microfluidics and lab-on-a-chip devices. In this work, we investigated the drop friction on lubricant-coated pillars by systematically varying pillar height and density. First, we measured the friction force on a moving drop using a cantilever force sensor that has ±0.1 μN sensitivity. This measurement shows that drop friction on tall dense pillars is comparable to drop friction on short pillars, a significant result that suggests the presence of a Landau-Levich-Derjaguin (LLD) film underneath the moving drop. Second, we validated the force measurement by estimating the lubricant layer thickness by using white-light interferometry. Third, we visualized the lubricant film underneath the moving drop using reflection interference contrast microscopy. The three independent diagnostic tools and measurement techniques complement each other and reaffirm that drops oleoplane on tall dense pillars, while they graze over the pillar tops in tall sparse pillars. The critical density that forces this transition to drop friction is ≈50%. Furthermore, the experimental results show that friction on microholes and micropillars is comparable when the solid fraction is the same. The results reported in this study contradict past studies that reported the absence of an oil layer on tall pillars. Besides improving current understanding, the insights gained from this work provide design guidelines for turning drop friction on-off on demand for microfluidics applications.

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Publication Details

Journal
ACS Applied Materials & Interfaces
Published
2025-10-08
DOI
https://doi.org/10.1021/acsami.5c08905
Primary Topic
Surface Modification and Superhydrophobicity
Type
article
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article

Drop Friction on Textured Lubricant-Coated Surfaces

Dan Daniel, Xiaoyu Chen, Biruk Teka Gidreta, Michał Remer et al.
ACS Applied Materials & Interfaces
Surface Modification and Superhydrophobicity
article

Drop Friction on Textured Lubricant-Coated Surfaces

Dan Daniel, Xiaoyu Chen, Biruk Teka Gidreta, Michał Remer, Solomon Adera, Xiaoguang Wang, Tanner Gaw
article en

Abstract

Understanding drop friction on textured surfaces has implications in microfluidics and lab-on-a-chip devices. In this work, we investigated the drop friction on lubricant-coated pillars by systematically varying pillar height and density. First, we measured the friction force on a moving drop using a cantilever force sensor that has ±0.1 μN sensitivity. This measurement shows that drop friction on tall dense pillars is comparable to drop friction on short pillars, a significant result that suggests the presence of a Landau-Levich-Derjaguin (LLD) film underneath the moving drop. Second, we validated the force measurement by estimating the lubricant layer thickness by using white-light interferometry. Third, we visualized the lubricant film underneath the moving drop using reflection interference contrast microscopy. The three independent diagnostic tools and measurement techniques complement each other and reaffirm that drops oleoplane on tall dense pillars, while they graze over the pillar tops in tall sparse pillars. The critical density that forces this transition to drop friction is ≈50%. Furthermore, the experimental results show that friction on microholes and micropillars is comparable when the solid fraction is the same. The results reported in this study contradict past studies that reported the absence of an oil layer on tall pillars. Besides improving current understanding, the insights gained from this work provide design guidelines for turning drop friction on-off on demand for microfluidics applications.

ACS Applied Materials & InterfacesVol. 17(43)
Warsaw University of Technology (PL), Michigan Department of Transportation (US), University of Michigan (US), The Ohio State University (US), King Abdullah University of Science and Technology (SA)
Openalex Percentile: Top 74%
Surface Modification and Superhydrophobicity
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