Neuromorphic Device Based on Material and Device Innovation toward Multimode and Multifunction

Neuromorphic devices, inspired by the human brain's efficiency and adaptability, hold great potential for artificial intelligence (AI) hardware to overcome the limitations of traditional von Neumann architecture. As a subclass, multimodal and multifunctional neuromorphic devices have recently gained a lot of attention due to their advantages in in‐sensor computing and sophisticated behaviors. In this review, recent advances in materials, device structures, and applications in this field are systematically presented. It includes optical, electrical, mechanical, and chemical sensing in multimodal neuromorphic device, which enable in‐sensor computing to minimize energy consumption and enhance real‐time decision‐making. The materials applied in this field such as phase‐change, 2D materials, and ferroelectrics are summarized for their roles in achieving synaptic plasticity, nonvolatile memory for multifunctional neuromorphic devices. Structural innovations, including reconfigurable, multi‐terminal, and 3D‐integrated designs, further optimize parallel processing and multifunctional integration. Besides, application scenarios of multimodal and multifunctional neuromorphic devices and their advantages for improving the efficiency of AI are reviewed. Finally, challenges in material stability and commercialization are discussed, it emphasizes the need for interdisciplinary efforts to bridge the gap. This review provides critical insights and future directions for developing brain‐inspired, energy‐efficient AI hardware.