Toward More Recyclable and Sustainable Lithium-Ion Batteries
The rapid rise of electric vehicles has driven significant advancements in lithium-ion battery (LIB) technology. However, the pursuit of higher power, longer lifespan, and greater capacity has often overshadowed critical factors such as recyclability, material sustainability, and environmental impact. To ensure the long-term viability of LIBs, future developments must strike a balance between performance and sustainability. This review advocates for the design of next-generation battery components using abundant, environmentally friendly, and sustainable materials that minimize reliance on intensive mining and refining processes. Key innovations include metal-free electrodes, nonmetallic current collectors, solid-state electrolytes, biodegradable components, anode-free configurations, and water-soluble binders for electrode fabrication. We provide a comprehensive assessment of recent progress in these areas, discuss challenges for practical implementation, and outline future directions for advancing these technologies. By offering a forward-looking perspective on innovative battery materials and designs, this review provides valuable insights into the sustainable evolution of LIBs.
Authors
- Jinxing Chen (ORCID: https://orcid.org/0000-0001-9254-7430)
- Guiling Wang (ORCID: https://orcid.org/0000-0002-2571-1760)
- Anthony U. Mu (ORCID: https://orcid.org/0000-0002-7689-4413)
- Panpan Xu (ORCID: https://orcid.org/0000-0001-7277-9920)
- Maura C. Appleberry (ORCID: https://orcid.org/0000-0001-9022-681X)
- Binglei Jiao
- Zheng Chen (ORCID: https://orcid.org/0000-0002-9186-4298)
- Feng Li (ORCID: https://orcid.org/0000-0003-0620-0639)
- Yinhai Liu
- Yuncheng Zhu
Institutions
- Harbin Engineering University (CN)
- Chinese Academy of Sciences (CN)
- University of California San Diego (US)
- Suzhou Institute of Nano-tech and Nano-bionics (CN)
- Institute of Molecular Functional Materials (CN)
- Centre for Sustainable Energy (GB)
- Centre de Coopération Universitaire Franco-Bavarois (DE)
- Division of Materials Science and Engineering (AU)
- Ministry of Education (ET)
Publication Details
- Journal
- ACS Applied Energy Materials
- Published
- 2025-10-04
- DOI
- https://doi.org/10.1021/acsaem.5c00605
- Primary Topic
- Extraction and Separation Processes
- Type
- article
- Field-Weighted Citation Impact
- 0.00