Topological magneto-optical Kerr effect without spin-orbit coupling in spin-compensated antiferromagnet

The magneto-optical Kerr effect (MOKE), the differential reflection of oppositely circularly polarized light, has traditionally been associated with relativistic spin-orbit coupling (SOC), which links a particle's spin with its orbital motion. In ferromagnets, large MOKE signals arise from the combination of magnetization and SOC, while in certain coplanar antiferromagnets, SOC-induced Berry curvature enables MOKE despite zero net magnetization. Theoretically, large MOKE can also arise in a broader class of magnetic materials with compensated spins, without relying on SOC - for example, in systems exhibiting real-space scalar spin chirality. The experimental verification has remained elusive. Here, we demonstrate such a SOC- and magnetization-free MOKE in the noncoplanar antiferromagnet Co<sub>1/3</sub>TaS<sub>2</sub>. Using a Sagnac interferometer microscope, we image domains of scalar spin chirality and their reversal. Our findings establish experimentally a new mechanism for generating large MOKE signals and position chiral spin textures in compensated magnets as a compelling platform for ultrafast, stray-field-immune opto-spintronic applications.

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Journal
Nature Communications
Published
2026-03-03
DOI
https://doi.org/10.1038/s41467-026-70238-0
Primary Topic
Magneto-Optical Properties and Applications
Type
article
Field-Weighted Citation Impact
0.00

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article

Topological magneto-optical Kerr effect without spin-orbit coupling in spin-compensated antiferromagnet

Yunpeng Gao, Kai Du, Sang‐Wook Cheong, Camron Farhang et al.
Nature Communications
Magneto-Optical Properties and Applications
article

Topological magneto-optical Kerr effect without spin-orbit coupling in spin-compensated antiferromagnet

Yunpeng Gao, Kai Du, Sang‐Wook Cheong, Camron Farhang, Jing Xia, Junjie Yang
article en

Abstract

The magneto-optical Kerr effect (MOKE), the differential reflection of oppositely circularly polarized light, has traditionally been associated with relativistic spin-orbit coupling (SOC), which links a particle's spin with its orbital motion. In ferromagnets, large MOKE signals arise from the combination of magnetization and SOC, while in certain coplanar antiferromagnets, SOC-induced Berry curvature enables MOKE despite zero net magnetization. Theoretically, large MOKE can also arise in a broader class of magnetic materials with compensated spins, without relying on SOC - for example, in systems exhibiting real-space scalar spin chirality. The experimental verification has remained elusive. Here, we demonstrate such a SOC- and magnetization-free MOKE in the noncoplanar antiferromagnet Co<sub>1/3</sub>TaS<sub>2</sub>. Using a Sagnac interferometer microscope, we image domains of scalar spin chirality and their reversal. Our findings establish experimentally a new mechanism for generating large MOKE signals and position chiral spin textures in compensated magnets as a compelling platform for ultrafast, stray-field-immune opto-spintronic applications.

Nature Communications
New Jersey Institute of Technology (US), University of California, Irvine (US)
National Science Foundation, U.S. Department of Energy, Gordon and Betty Moore Foundation, UC Irvine Materials Research Institute, University of California, Irvine, Division of Materials Research
Openalex Percentile: Top 100%
Magneto-Optical Properties and Applications
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Topological magneto-optical Kerr effect without spin-orbit coupling in spin-compensated antiferromagnet — Yunpeng Gao, Kai Du, et al. · Nature Communications (2026) | TGRS Research Map | TGRS