Strong springtime increase of ice-nucleating particle concentration in the Rocky Mountains

Abstract. Ice nucleating particles (INPs) exert a substantial impact on radiative properties and lifetimes of mixed-phase clouds and can modulate their precipitation efficiency. Advancing our understanding of the abundance and properties of INPs is essential to elucidate how clouds change in a warming climate. We conducted INP measurements at the Storm Peak Laboratory (3200 m a.s.l.), in the Rocky Mountains (CO, USA) during two field campaigns in 2021/2022 and in 2025. INP concentrations were continuously measured with the Portable Ice Nucleation Experiment between −22 and −32 °C. INP concentrations were remarkably similar during the two campaigns and followed a seasonal pattern. Lowest concentrations were observed during winter, with median January values falling below 10 INP stdL−1 at T > −26 °C. In spring, median INP concentrations increased by approximately one order of magnitude. Springtime is associated with increased dust concentrations in the Western United States, and back trajectories revealed regional and local dust regions as INP sources. As climate change is expected to intensify the influence of dust sources from deserts and semi-arid regions, this might impact INP concentrations. Moreover, INP sizes were investigated by ranked correlation coefficient analysis of parallel measurements of super-micrometer particles, the application of a novel setup of a pumped-counterflow virtual impactor downstream of PINE to analyze the sizes of ice residuals, and alternated INP measurements at a 1 µm impactor. Overall, super-micrometer particles were found to contribute significantly to the INP population throughout the entire campaign, with a reduced importance during winter.