Exact Large-Scale Correlations in Diffusive Systems with General Interactions

Characterizing the statistical properties of classical interacting particle systems is a long-standing question. For Brownian particles, the microscopic density obeys a stochastic evolution equation, known as the Dean-Kawasaki equation. This equation remains mostly formal and linearization (or higher-order expansions) is required to obtain explicit expressions for physical observables, with a range of validity not easily defined. Here, by combining macroscopic fluctuation theory with equilibrium statistical mechanics, we provide a systematic alternative to the Dean-Kawasaki framework to characterize large-scale correlations. This approach enables us to obtain explicit and exact results for the large-scale behavior of dynamical observables such as tracer cumulants and bath-tracer correlations in one dimension, both in and out of equilibrium. In particular, we reveal a generic nonmonotonic spatial structure in the response of the bath following a temperature quench. Our approach applies to a broad class of interaction potentials and extends naturally to higher dimensions.

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Publication Details

Journal
Physical Review Letters
Published
2025-09-25
DOI
https://doi.org/10.1103/gwdh-3vqm
Primary Topic
Advanced Thermodynamics and Statistical Mechanics
Type
article
Field-Weighted Citation Impact
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article

Exact Large-Scale Correlations in Diffusive Systems with General Interactions

Olivier Bénichou, Aurélien Grabsch, Davide Venturelli
Physical Review Letters
Advanced Thermodynamics and Statistical Mechanics
article

Exact Large-Scale Correlations in Diffusive Systems with General Interactions

Olivier Bénichou, Aurélien Grabsch, Davide Venturelli
article en

Abstract

Characterizing the statistical properties of classical interacting particle systems is a long-standing question. For Brownian particles, the microscopic density obeys a stochastic evolution equation, known as the Dean-Kawasaki equation. This equation remains mostly formal and linearization (or higher-order expansions) is required to obtain explicit expressions for physical observables, with a range of validity not easily defined. Here, by combining macroscopic fluctuation theory with equilibrium statistical mechanics, we provide a systematic alternative to the Dean-Kawasaki framework to characterize large-scale correlations. This approach enables us to obtain explicit and exact results for the large-scale behavior of dynamical observables such as tracer cumulants and bath-tracer correlations in one dimension, both in and out of equilibrium. In particular, we reveal a generic nonmonotonic spatial structure in the response of the bath following a temperature quench. Our approach applies to a broad class of interaction potentials and extends naturally to higher dimensions.

Physical Review LettersVol. 135(13)
Sorbonne Université (FR), Laboratoire Jean Perrin (FR), Laboratoire de Physique Théorique de la Matière Condensée (FR), Laboratoire Médiations (FR)
Openalex Percentile: Top 79%
Advanced Thermodynamics and Statistical Mechanics
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