Hyperspectral microscopy with Computational field-resolved Coherent anti-Stokes Raman Scattering

High-dimensional statistics of CARS leads to high time and storage consumption. We introduced a computational field-resolved CARS method for hyperspectral microscopy of materials and biological samples. Compared to traditional broadband CARS, our proposed method provides access to the spectral phase, thereby enabling quantitative chemical imaging. The reconstruction can be achieved within 10 minutes.