Continuous-time multifarious systems. II. Non-reciprocal multifarious self-organization

In the context of self-assembly, where complex structures can be assembled from smaller units, it is desirable to devise strategies toward disassembly and reassembly processes that reuse the constituent parts. A non-reciprocal multifarious self-organization strategy has been recently introduced and shown to have the capacity to exhibit this complex property. In this work, we study the model using continuous-time Gillespie simulations and compare the results against discrete-time Monte Carlo simulations investigated previously. Furthermore, using the continuous-time simulations, we explore important features in our system, namely, the nucleation time and interface growth velocity, which comprise the timescale of shape-shifting. We develop analytical calculations for the associated timescales and compare the results to those measured in simulations, allowing us to pin down the key mechanisms behind the observed timescales at different parameter values.

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Publication Details

Journal
The Journal of Chemical Physics
Published
2025-09-23
DOI
https://doi.org/10.1063/5.0284977
Citations
2
Primary Topic
Theoretical and Computational Physics
Type
article
Field-Weighted Citation Impact
2.52
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article

Continuous-time multifarious systems. II. Non-reciprocal multifarious self-organization

Saeed Osat, Ramin Golestanian, Jakob Metson
2 citations
The Journal of Chemical Physics
Theoretical and Computational Physics
2.52
article

Continuous-time multifarious systems. II. Non-reciprocal multifarious self-organization

Saeed Osat, Ramin Golestanian, Jakob Metson
article en
2 citations

Abstract

In the context of self-assembly, where complex structures can be assembled from smaller units, it is desirable to devise strategies toward disassembly and reassembly processes that reuse the constituent parts. A non-reciprocal multifarious self-organization strategy has been recently introduced and shown to have the capacity to exhibit this complex property. In this work, we study the model using continuous-time Gillespie simulations and compare the results against discrete-time Monte Carlo simulations investigated previously. Furthermore, using the continuous-time simulations, we explore important features in our system, namely, the nucleation time and interface growth velocity, which comprise the timescale of shape-shifting. We develop analytical calculations for the associated timescales and compare the results to those measured in simulations, allowing us to pin down the key mechanisms behind the observed timescales at different parameter values.

The Journal of Chemical PhysicsVol. 163(12)
Center for Theoretical Physics (PL), University of Oxford (GB), Max Planck Institute for Dynamics and Self-Organization (DE)
Openalex Percentile: Top 10%
Theoretical and Computational Physics
2.52
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