Ultrafast Electron Temperature Dynamics in Spintronic Terahertz Emitters Studied by Optical-Pump Terahertz-Probe Spectroscopy

Spintronic terahertz emitters (STEs) pumped by femtosecond lasers have become a widely used source of broadband terahertz radiation. However, the strength of the emitted field is limited in part by the optical damage threshold at the pump wavelength. Thermal management of STEs can be improved by understanding electron temperature relaxation in the spintronic metal layer. Here, we present a measurement of electron temperature dynamics on a picosecond time scale using optical-pump terahertz-probe spectroscopy. We observe that the optical pump induces a change in terahertz transmission through the STE. By analyzing the resulting signal with a two-temperature model, we extract the dynamic electron temperature of the STE. This approach offers an advantage over other methods by avoiding additional heating of the sample by the probe pulse, making it particularly suitable for studying cumulative heating effects, which are believed to contribute to optical damage under MHz repetition rate pumping.

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Publication Details

Journal
ACS Photonics
Published
2025-08-15
DOI
https://doi.org/10.1021/acsphotonics.5c01419
Citations
1
Primary Topic
Terahertz technology and applications
Type
article
Field-Weighted Citation Impact
0.73

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article

Ultrafast Electron Temperature Dynamics in Spintronic Terahertz Emitters Studied by Optical-Pump Terahertz-Probe Spectroscopy

Johanna Kölbel, Felix Selz, Georg von Freymann, Daniel M. Mittleman et al.
1 citations
ACS Photonics
Terahertz technology and applications
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article

Ultrafast Electron Temperature Dynamics in Spintronic Terahertz Emitters Studied by Optical-Pump Terahertz-Probe Spectroscopy

Johanna Kölbel, Felix Selz, Georg von Freymann, Daniel M. Mittleman, Felix Paries, Daniel Molter
article en
1 citations

Abstract

Spintronic terahertz emitters (STEs) pumped by femtosecond lasers have become a widely used source of broadband terahertz radiation. However, the strength of the emitted field is limited in part by the optical damage threshold at the pump wavelength. Thermal management of STEs can be improved by understanding electron temperature relaxation in the spintronic metal layer. Here, we present a measurement of electron temperature dynamics on a picosecond time scale using optical-pump terahertz-probe spectroscopy. We observe that the optical pump induces a change in terahertz transmission through the STE. By analyzing the resulting signal with a two-temperature model, we extract the dynamic electron temperature of the STE. This approach offers an advantage over other methods by avoiding additional heating of the sample by the probe pulse, making it particularly suitable for studying cumulative heating effects, which are believed to contribute to optical damage under MHz repetition rate pumping.

ACS PhotonicsVol. 12(9)
University of Freiburg (DE), John Brown University (US), Brown University (US), Fraunhofer Institute for Industrial Mathematics (DE), FZU ‒ Institute of Physics of the Academy of Sciences of the Czech Republic (CZ), Rheinland-Pfälzische Technische Universität Kaiserslautern-Landau (DE)
National Science Foundation, Deutsche Forschungsgemeinschaft, Studienstiftung des Deutschen Volkes, Division of Electrical, Communications and Cyber Systems
Openalex Percentile: Top 23%
Terahertz technology and applications
0.73
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