Mean-field mixed quantum-classical approach for many-body quantum dynamics of exciton polaritons

Coupling material excitations to photons inside optical cavities has been experimentally shown to give rise to a wide range of exotic quantum phenomena, and such light--matter hybrid systems have been proposed as versatile platforms for developing quantum devices. However, the theoretical understanding of the interplay between phonon-induced disorder and nonlinear many-body interactions, central to the dynamics of these systems, remains unclear, as incorporating these contributions into direct quantum dynamical simulations is highly challenging. To address this, the authors develop here a mean-field many-body mixed quantum--classical approach, in which the nuclei are propagated quasiclassically while the electronic and photonic degrees of freedom evolve under a nonlinear Schr"odinger equation that incorporates many-body effects at the mean-field level. Using this framework, the authors demonstrate that nonlinear interactions and the total number of excitations can be tuned to enhance quantum coherence in light--matter systems and enable enhanced exciton transport in materials placed inside optical cavities.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-09-03
DOI
https://doi.org/10.1103/m53p-sfc5
Citations
3
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
3.74
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Mean-field mixed quantum-classical approach for many-body quantum dynamics of exciton polaritons

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article

Mean-field mixed quantum-classical approach for many-body quantum dynamics of exciton polaritons

Sachith Wickramasinghe, Saeed Rahmanian Koshkaki, Arkajit Mandal, Pritha Ghosh, Arshath Manjalingal
article en
3 citations

Abstract

Coupling material excitations to photons inside optical cavities has been experimentally shown to give rise to a wide range of exotic quantum phenomena, and such light--matter hybrid systems have been proposed as versatile platforms for developing quantum devices. However, the theoretical understanding of the interplay between phonon-induced disorder and nonlinear many-body interactions, central to the dynamics of these systems, remains unclear, as incorporating these contributions into direct quantum dynamical simulations is highly challenging. To address this, the authors develop here a mean-field many-body mixed quantum--classical approach, in which the nuclei are propagated quasiclassically while the electronic and photonic degrees of freedom evolve under a nonlinear Schr\"odinger equation that incorporates many-body effects at the mean-field level. Using this framework, the authors demonstrate that nonlinear interactions and the total number of excitations can be tuned to enhance quantum coherence in light--matter systems and enable enhanced exciton transport in materials placed inside optical cavities.

Physical review. B./Physical review. BVol. 112(10)
Mitchell Institute (US), Texas A&M University (US)
Openalex Percentile: Top 6%
Strong Light-Matter Interactions
3.74
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