Nonlinear refractive index measurements of solids and the impact of B-integral on the phase of generated high-order harmonics

We present an interferometric method that employs a birefringent common-path interferometer to measure absolute nonlinear refractive indices in 5 mm thick CaF₂, SiO₂, NBK-7 and KBr for femtosecond pulses at 804-nm center wavelength. The measured nonlinear refractive indices are found to be in agreement with previous literature, over a broad range of pulse energies. In addition, we show and highlight the importance of thorough B-integral characterization when using this birefringent common-path interferometer for high-harmonic generation driven extreme-ultraviolet interferometry. The accumulated third-order nonlinear phase is shown to have significant impact on the harmonic phase after up-conversion to higher orders, but can be accounted for if correctly characterized.

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Publication Details

Published
2025-09-22
DOI
https://doi.org/10.1364/opticaopen.30172501
Primary Topic
Optical and Acousto-Optic Technologies
Type
article
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article

Nonlinear refractive index measurements of solids and the impact of B-integral on the phase of generated high-order harmonics

Nataliia Kuzkova, Peter M. Kraus, Roy van der Linden
Optical and Acousto-Optic Technologies
article

Nonlinear refractive index measurements of solids and the impact of B-integral on the phase of generated high-order harmonics

Nataliia Kuzkova, Peter M. Kraus, Roy van der Linden
article en

Abstract

We present an interferometric method that employs a birefringent common-path interferometer to measure absolute nonlinear refractive indices in 5 mm thick CaF₂, SiO₂, NBK-7 and KBr for femtosecond pulses at 804-nm center wavelength. The measured nonlinear refractive indices are found to be in agreement with previous literature, over a broad range of pulse energies. In addition, we show and highlight the importance of thorough B-integral characterization when using this birefringent common-path interferometer for high-harmonic generation driven extreme-ultraviolet interferometry. The accumulated third-order nonlinear phase is shown to have significant impact on the harmonic phase after up-conversion to higher orders, but can be accounted for if correctly characterized.

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Optical and Acousto-Optic Technologies
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