Dzyaloshinskii–Moriya Interaction in Fe<sub>5</sub>GeTe<sub>2</sub> Epitaxial Thin Films
van der Waals ferromagnets, such as Fe<sub>5</sub>GeTe<sub>2</sub>, offer a promising platform for spintronic devices based on chiral magnetic textures, provided a significant Dzyaloshinskii-Moriya interaction (DMI) can be induced to stabilize the textures. Here, we directly measure DMI in epitaxial Fe<sub>5</sub>GeTe<sub>2</sub> thin films using Brillouin light scattering spectroscopy and observe a consistent DMI (<i>D</i> = 0.04 mJ/m<sup>2</sup>) across various thicknesses. Its weak thickness dependence, combined with the nominally symmetric film interfaces, suggests a bulk origin. Although we do not determine the microscopic mechanism, our findings are compatible with <i>ab initio</i> calculations linking DMI to partial ordering of Fe split sites. Additionally, we find a low magnetic dissipation (α < 0.02). The observed DMI, which could be further enhanced by optimizing the Fe site ordering, combined with low dissipation, makes Fe<sub>5</sub>GeTe<sub>2</sub> a strong candidate for exploring the dynamics of chiral magnetic textures in two-dimensional materials.
Authors
- A. Marty (ORCID: https://orcid.org/0000-0001-5709-6945)
- A. Mougin (ORCID: https://orcid.org/0000-0001-8607-0154)
- Antoine Pascaud (ORCID: https://orcid.org/0000-0002-4092-9493)
- Frédéric Bonell (ORCID: https://orcid.org/0000-0001-7296-0404)
- A. Thiaville (ORCID: https://orcid.org/0000-0003-0140-9740)
- Vincent Polewczyk (ORCID: https://orcid.org/0000-0003-0932-6376)
- J. Sampaio (ORCID: https://orcid.org/0000-0002-0460-3664)
- Edgar Quero
Institutions
- Centre National de la Recherche Scientifique (FR)
- Commissariat à l'Énergie Atomique et aux Énergies Alternatives (FR)
- Université Paris-Saclay (FR)
- Laboratoire de physique des Solides (FR)
- CEA Grenoble (FR)
- Spintronique et Technologie des Composants (FR)
- Université Grenoble Alpes (FR)
Publication Details
- Journal
- Nano Letters
- Published
- 2025-09-19
- DOI
- https://doi.org/10.1021/acs.nanolett.5c03547
- Citations
- 3
- Primary Topic
- Magnetic properties of thin films
- Type
- article
- Field-Weighted Citation Impact
- 3.74