Polycrystalline MAPbI <sub>3</sub> AC-bias direct x-ray detectors for 3D reconstruction
Metal halide perovskites offer exceptional sensitivity for direct x-ray detection through direct current (DC) signals, but the DC bias-induced ion migration poses substantial challenges to their signal consistency and operational stability. In this work, we propose a capacitance signal-based imaging strategy that uses an alternating current (AC) bias to suppress ion migration and eliminate nonlinear responses. A quantitative correlation between capacitance changes and x-ray dose rate is established, enabling stable, high-resolution imaging. Using this method, we achieve three-dimensional internal structure reconstruction with a simple single-pixel detector. This approach overcomes intrinsic material limitations and enhances signal reliability, providing a promising pathway toward the commercialization of low-cost, high-performance perovskite-based x-ray imaging and computed tomography systems.
Authors
- Ziyao Zhu (ORCID: https://orcid.org/0000-0003-4375-2133)
- Sheng Gao (ORCID: https://orcid.org/0000-0003-0249-3462)
- Wenjun Liu (ORCID: https://orcid.org/0000-0001-8881-7039)
- Yunlong Li (ORCID: https://orcid.org/0000-0002-7193-7322)
- Xiumin Xu (ORCID: https://orcid.org/0000-0001-7902-3050)
- Jun Wang (ORCID: https://orcid.org/0000-0002-3242-6570)
- Bo Zhao
- Yang He (ORCID: https://orcid.org/0000-0002-8530-9132)
Institutions
- Anhui University (CN)
- Chinese Academy of Sciences (CN)
- Education University of Hong Kong (HK)
- Shenzhen Institutes of Advanced Technology (CN)
Publication Details
- Journal
- Science Advances
- Published
- 2025-09-19
- DOI
- https://doi.org/10.1126/sciadv.adx8785
- Primary Topic
- Perovskite Materials and Applications
- Type
- article
- Field-Weighted Citation Impact
- 0.00