Polycrystalline MAPbI <sub>3</sub> AC-bias direct x-ray detectors for 3D reconstruction

Metal halide perovskites offer exceptional sensitivity for direct x-ray detection through direct current (DC) signals, but the DC bias-induced ion migration poses substantial challenges to their signal consistency and operational stability. In this work, we propose a capacitance signal-based imaging strategy that uses an alternating current (AC) bias to suppress ion migration and eliminate nonlinear responses. A quantitative correlation between capacitance changes and x-ray dose rate is established, enabling stable, high-resolution imaging. Using this method, we achieve three-dimensional internal structure reconstruction with a simple single-pixel detector. This approach overcomes intrinsic material limitations and enhances signal reliability, providing a promising pathway toward the commercialization of low-cost, high-performance perovskite-based x-ray imaging and computed tomography systems.

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Publication Details

Journal
Science Advances
Published
2025-09-19
DOI
https://doi.org/10.1126/sciadv.adx8785
Primary Topic
Perovskite Materials and Applications
Type
article
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article

Polycrystalline MAPbI 3 AC-bias direct x-ray detectors for 3D reconstruction

Ziyao Zhu, Sheng Gao, Wenjun Liu, Yunlong Li et al.
Science Advances
Perovskite Materials and Applications
article

Polycrystalline MAPbI 3 AC-bias direct x-ray detectors for 3D reconstruction

Ziyao Zhu, Sheng Gao, Wenjun Liu, Yunlong Li, Xiumin Xu, Jun Wang, Bo Zhao, Yang He
article en

Abstract

Metal halide perovskites offer exceptional sensitivity for direct x-ray detection through direct current (DC) signals, but the DC bias-induced ion migration poses substantial challenges to their signal consistency and operational stability. In this work, we propose a capacitance signal-based imaging strategy that uses an alternating current (AC) bias to suppress ion migration and eliminate nonlinear responses. A quantitative correlation between capacitance changes and x-ray dose rate is established, enabling stable, high-resolution imaging. Using this method, we achieve three-dimensional internal structure reconstruction with a simple single-pixel detector. This approach overcomes intrinsic material limitations and enhances signal reliability, providing a promising pathway toward the commercialization of low-cost, high-performance perovskite-based x-ray imaging and computed tomography systems.

Science AdvancesVol. 11(38)
Anhui University (CN), Chinese Academy of Sciences (CN), Education University of Hong Kong (HK), Shenzhen Institutes of Advanced Technology (CN)
Openalex Percentile: Top 75%
Perovskite Materials and Applications
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Polycrystalline MAPbI <sub>3</sub> AC-bias direct x-ray detectors for 3D reconstruction — Ziyao Zhu, Sheng Gao, et al. · Science Advances (2025) | TGRS Research Map | TGRS