Anomalous lattice relaxation dynamics in optimally doped <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>La</mml:mi><mml:mrow><mml:mn>2</mml:mn><mml:mo>−</mml:mo><mml:mi>x</mml:mi></mml:mrow></mml:msub><mml:msub><
The atomic lattice plays a critical role in the emergence of high-<a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:msub><a:mi>T</a:mi><a:mi>c</a:mi></a:msub></a:math> superconductivity in cuprates. While the dynamics associated with electron-lattice coupling typically unfold on picosecond-to-femtosecond timescales, we present an x-ray photon correlation spectroscopy investigation on an optimally doped La-based cuprate that reveals a strong response of kilosecond-scale lattice relaxation dynamics to the superconducting state. Notably, an anomaly emerges around <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"><b:msub><b:mi>T</b:mi><b:mi>c</b:mi></b:msub></b:math>: upon cooling into the superconducting state, the average atomic relaxation lifetime decreases, i.e., dynamics accelerate. This indicates a significant change in the local disorder-induced strain field dynamics at the superconducting transition, highlighting a remarkable coupling between superconductivity and the lattice on quasistatic timescales.
Authors
- L. Shen (ORCID: https://orcid.org/0000-0002-2121-2585)
- Ross Arthur
- Joshua J. Turner (ORCID: https://orcid.org/0000-0002-2106-7955)
- Vivek Thampy (ORCID: https://orcid.org/0000-0003-3983-3109)
- Michael Sprung (ORCID: https://orcid.org/0000-0003-2396-3304)
- Zhe Ren (ORCID: https://orcid.org/0000-0003-2446-6772)
- Annika Stellhorn (ORCID: https://orcid.org/0000-0003-2868-657X)
- A. Alshemi (ORCID: https://orcid.org/0000-0003-0271-5299)
- Alexander N. Petsch (ORCID: https://orcid.org/0000-0002-7597-9626)
- S. M. Hayden (ORCID: https://orcid.org/0000-0002-3209-027X)
- E. Blackburn (ORCID: https://orcid.org/0000-0002-5119-6053)
- Zach Porter (ORCID: https://orcid.org/0000-0002-2945-9558)
- Fabian Westermeier (ORCID: https://orcid.org/0000-0003-0696-206X)
- Hasan Yavaş (ORCID: https://orcid.org/0000-0002-8940-3556)
- Aidan Israelski (ORCID: https://orcid.org/0000-0003-1540-4377)
- Peng Cheng (ORCID: https://orcid.org/0000-0002-9267-1789)
Institutions
- Lund University (SE)
- Deutsches Elektronen-Synchrotron DESY (DE)
- SLAC National Accelerator Laboratory (US)
- University of Bristol (GB)
- Stanford University (US)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-09-18
- DOI
- https://doi.org/10.1103/9sg4-52qz
- Primary Topic
- Physics of Superconductivity and Magnetism
- Type
- article
- Field-Weighted Citation Impact
- 0.00