Unfolding the kagome lattice to improve understanding of ARPES in CoSn

Metallic kagome lattices are attracting significant attention as they provide a platform to explore the interplay between topology and magnetism. Angle-resolved photoemission spectroscopy (ARPES) plays a key role in unraveling their electronic structure. However, the analysis is often challenging due to the presence of multiple bands near the Fermi level. Indeed, each orbital generates three bands in a kagome lattice due to its three sites motif, which soon becomes complicated if many orbitals are present. To address this complexity, using ARPES matrix elements can be highly beneficial. First, band symmetry can be determined through selection rules based on light polarization. We emphasize that, in kagome lattices, as in all multisite lattices, symmetry of the Bloch state is not only determined by the orbital character but also by the relative phase between the three sublattices. Additionally, interference between the three sublattices leads to a strong modulation of ARPES intensity across neighboring Brillouin zones. We show how unfolded band calculations capture these modulations, helping with band identification. We apply these ideas to CoSn, whose simple structure retains the key features of a kagome lattice. Using polarization dependent ARPES in several Brillouin zones, we isolate the dispersion of each band and discuss novel correlation effects, selectively renormalizing the bands crossing the Fermi level and shifting the others.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-08-25
DOI
https://doi.org/10.1103/5rpf-sd26
Primary Topic
Electronic and Structural Properties of Oxides
Type
article
Field-Weighted Citation Impact
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article

Unfolding the kagome lattice to improve understanding of ARPES in CoSn

Oleg Rubel, F. Bertran, V. Brouet, Patrick Le Fèvre et al.
Physical review. B./Physical review. B
Electronic and Structural Properties of Oxides
article

Unfolding the kagome lattice to improve understanding of ARPES in CoSn

Oleg Rubel, F. Bertran, V. Brouet, Patrick Le Fèvre, Aaditya Vedant
article en

Abstract

Metallic kagome lattices are attracting significant attention as they provide a platform to explore the interplay between topology and magnetism. Angle-resolved photoemission spectroscopy (ARPES) plays a key role in unraveling their electronic structure. However, the analysis is often challenging due to the presence of multiple bands near the Fermi level. Indeed, each orbital generates three bands in a kagome lattice due to its three sites motif, which soon becomes complicated if many orbitals are present. To address this complexity, using ARPES matrix elements can be highly beneficial. First, band symmetry can be determined through selection rules based on light polarization. We emphasize that, in kagome lattices, as in all multisite lattices, symmetry of the Bloch state is not only determined by the orbital character but also by the relative phase between the three sublattices. Additionally, interference between the three sublattices leads to a strong modulation of ARPES intensity across neighboring Brillouin zones. We show how unfolded band calculations capture these modulations, helping with band identification. We apply these ideas to CoSn, whose simple structure retains the key features of a kagome lattice. Using polarization dependent ARPES in several Brillouin zones, we isolate the dispersion of each band and discuss novel correlation effects, selectively renormalizing the bands crossing the Fermi level and shifting the others.

Physical review. B./Physical review. BVol. 112(11)
Université Paris-Saclay (FR), Synchrotron soleil (FR), McMaster University (CA)
Openalex Percentile: Top 81%
Electronic and Structural Properties of Oxides
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