Photoinduced non-reciprocal magnetism

Out of equilibrium, the action-reaction symmetry of interactions is often broken, leading to the emergence of various collective phenomena with no equilibrium counterparts. Although ubiquitous in classical active systems, implementing such non-reciprocal interactions in solid-state systems has remained challenging, as known quantum schemes require precise single-site control. Here, we propose a dissipation-engineering protocol that induces non-reciprocal interactions in solid-state platforms with light, which we expect to be achievable with state-of-the-art experimental techniques. Focusing on magnetic metals, we show microscopically that a light injection that introduces a decay channel to a virtually excited state gives rise to non-reciprocal interactions between localized spins, resulting in chase-and-runaway dynamics. Applying our scheme to layered ferromagnets, we show that a non-reciprocal phase transition to a many-body time-dependent chiral phase occurs. Our work paves the way to bring solid-state systems to the realm of non-reciprocal science, providing yet another possibility to control quantum matter with light.

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Publication Details

Journal
Nature Communications
Published
2025-09-18
DOI
https://doi.org/10.1038/s41467-025-62707-9
Citations
3
Primary Topic
Magnetic properties of thin films
Type
article
Field-Weighted Citation Impact
3.74

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article

Photoinduced non-reciprocal magnetism

Daiki Ootsuki, Rina Tazai, Ryo Hanai
3 citations
Nature Communications
Magnetic properties of thin films
3.74
article

Photoinduced non-reciprocal magnetism

Daiki Ootsuki, Rina Tazai, Ryo Hanai
article en
3 citations

Abstract

Out of equilibrium, the action-reaction symmetry of interactions is often broken, leading to the emergence of various collective phenomena with no equilibrium counterparts. Although ubiquitous in classical active systems, implementing such non-reciprocal interactions in solid-state systems has remained challenging, as known quantum schemes require precise single-site control. Here, we propose a dissipation-engineering protocol that induces non-reciprocal interactions in solid-state platforms with light, which we expect to be achievable with state-of-the-art experimental techniques. Focusing on magnetic metals, we show microscopically that a light injection that introduces a decay channel to a virtually excited state gives rise to non-reciprocal interactions between localized spins, resulting in chase-and-runaway dynamics. Applying our scheme to layered ferromagnets, we show that a non-reciprocal phase transition to a many-body time-dependent chiral phase occurs. Our work paves the way to bring solid-state systems to the realm of non-reciprocal science, providing yet another possibility to control quantum matter with light.

Nature CommunicationsVol. 16(1)
Tokyo Institute of Technology (JP), Okayama University of Science (JP), Kyoto University (JP)
National Research Foundation, Japan Society for the Promotion of Science
Openalex Percentile: Top 6%
Magnetic properties of thin films
3.74
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