Phase-sensitive Surface Second-harmonic Generation of Topological Dirac Semimetal

We report anomalously strong, surface-specific, purely out-of-plane optical nonlinearity in PdTe 2 Dirac semimetal through polarization-dependent heterodyne-interferometric rotational-anisotropic second-harmonic generation. This strong nonlinearity is correlated to the topological surface states via surface and orbital-projected band calculations.

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Publication Details

Published
2025-01-01
DOI
https://doi.org/10.1364/cleo_fs.2025.ff135_5
Primary Topic
Topological Materials and Phenomena
Type
article
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article

Phase-sensitive Surface Second-harmonic Generation of Topological Dirac Semimetal

C. S. Lue, Hsin Lin, Po-Yuan Yang, Ching-Hang Chien et al.
Topological Materials and Phenomena
article

Phase-sensitive Surface Second-harmonic Generation of Topological Dirac Semimetal

C. S. Lue, Hsin Lin, Po-Yuan Yang, Ching-Hang Chien, Yu‐Chieh Wen, Yao-Jui Chan, Syed Mohammed Faizanuddin, Tay-Rong Chang, Chia‐Nung Kuo
article en

Abstract

We report anomalously strong, surface-specific, purely out-of-plane optical nonlinearity in PdTe 2 Dirac semimetal through polarization-dependent heterodyne-interferometric rotational-anisotropic second-harmonic generation. This strong nonlinearity is correlated to the topological surface states via surface and orbital-projected band calculations.

Openalex Percentile: Top 80%
Topological Materials and Phenomena
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