Spatially resolved <i>operando</i> X-ray diffraction for mapping heterogeneities in Li-ion single-layer pouch cells
The electrochemical degradation of Li-ion batteries occurs over different spatial and temporal scales. This work demonstrates how <i>operando</i> synchrotron X-ray diffraction can be used to study degradation in Li-ion battery materials by mapping component-specific crystallographic structure evolution across a single-layer pouch full cell in real-time, enabling quantification of structural degradation processes in Li-ion battery cells from the atomic to macroscopic scale.
Authors
- Serena A. Cussen (ORCID: https://orcid.org/0000-0002-9303-4220)
- Simon D. M. Jacques (ORCID: https://orcid.org/0000-0002-7275-5272)
- Louis F. J. Piper (ORCID: https://orcid.org/0000-0002-3421-3210)
- Andrew M. Beale (ORCID: https://orcid.org/0000-0002-0923-1433)
- Innes McClelland (ORCID: https://orcid.org/0000-0001-9821-715X)
- Navneet Kaur
- Ashok Sreekumar Menon (ORCID: https://orcid.org/0000-0001-8148-8615)
- Stephen W. T. Price (ORCID: https://orcid.org/0000-0002-5329-4351)
- Nickil Shah (ORCID: https://orcid.org/0000-0002-4188-1209)
- Muhammad Ans (ORCID: https://orcid.org/0000-0002-1312-3304)
- Pol Sallés Perramon
Institutions
- University College Dublin (IE)
- Rutherford Appleton Laboratory (GB)
- University of Warwick (GB)
- Research Complex at Harwell (GB)
- The Faraday Institution (GB)
- University College London (GB)
Publication Details
- Journal
- Chemical Communications
- Published
- 2025-01-01
- DOI
- https://doi.org/10.1039/d5cc02935j
- Citations
- 3
- Primary Topic
- Advancements in Battery Materials
- Type
- article
- Field-Weighted Citation Impact
- 2.19