Cavity exciton-polariton condensation in perovskite quantum dots at room-temperature

In this study, we demonstrate room-temperature polariton condensation using a thin film of monodisperse colloidal CsPbBr₃ quantum dots embedded in a tunable optical microcavity. The cavity incorporates a Gaussian-shaped deformation, which functions as a wavelength-scale potential well for polaritons. Under pulsed optical excitation, we observe key signatures of polariton condensation, including a characteristic superlinear increase in emission intensity, linewidth narrowing, energy blueshift, and extended temporal coherence. These findings highlight the potential of perovskite-based colloidal quantum dots, renowned for their outstanding optical properties and high tunability, as a favourable platform for next-generation polaritonic devices.

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Published
2025-09-16
DOI
https://doi.org/10.1117/12.3066289
Primary Topic
Strong Light-Matter Interactions
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article
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article

Cavity exciton-polariton condensation in perovskite quantum dots at room-temperature

Ioannis Georgakilas
Strong Light-Matter Interactions
article

Cavity exciton-polariton condensation in perovskite quantum dots at room-temperature

Ioannis Georgakilas
article en

Abstract

In this study, we demonstrate room-temperature polariton condensation using a thin film of monodisperse colloidal CsPbBr₃ quantum dots embedded in a tunable optical microcavity. The cavity incorporates a Gaussian-shaped deformation, which functions as a wavelength-scale potential well for polaritons. Under pulsed optical excitation, we observe key signatures of polariton condensation, including a characteristic superlinear increase in emission intensity, linewidth narrowing, energy blueshift, and extended temporal coherence. These findings highlight the potential of perovskite-based colloidal quantum dots, renowned for their outstanding optical properties and high tunability, as a favourable platform for next-generation polaritonic devices.

IBM Research - Zurich (CH)
Openalex Percentile: Top 81%
Strong Light-Matter Interactions
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