Non-equilibrium dynamics of disordered bead-spring networks with active forces

We investigate, using Langevin dynamics simulations, the Rouse-type dynamics of active harmonic bead-spring percolation clusters of square and triangular lattices. Two types of active stochastic forces, modeled as a random telegraph process with correlation time τ, are considered: force monopoles, acting on individual nodes in random directions, and force dipoles, where extensile or contractile forces act between pairs of nodes. For force monopoles, a dynamical steady state is reached where the network is dynamically swollen and the mean square displacement (MSD) shows sub-diffusive behavior at t > τ, MSD ∼ tν, with ν=1-ds2 where ds is the spectral dimension, in accord with a previously advanced general analytic theory. In contrast, dipolar forces require diverging times to reach steady state and lead to network shrinkage. Within a quasi-steady-state approximation, the MSD is found to saturate at the same temporal regime t > τ, which is followed by ballistic-like and/or diffusive behaviors. We further extend our study of dipolar forces to dilution regimes above the isostatic threshold, also known as "rigidity percolation". Here, weak dipolar forces effectively do not shrink the network in steady state. Instead, they induce "rotational swimming" of the network. Yet, for the triangular lattice, an incipient discontinuous collapse transition occurs above a critical force amplitude value. Conversely, we find a continuous crossover to a collapsed state for the non-diluted square lattice, resulting from its marginal stability. We suggest that disordered solids be poised above the isostatic point to be stable against active dipolar forces, provided that the dynamical persistent length remains lower than the spring rest length.

Authors

Institutions

Publication Details

Journal
The Journal of Chemical Physics
Published
2025-09-15
DOI
https://doi.org/10.1063/5.0278300
Primary Topic
Dynamics and Control of Mechanical Systems
Type
article
Field-Weighted Citation Impact
0.00
Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Non-equilibrium dynamics of disordered bead-spring networks with active forces

Debjyoti Majumdar, Rony Granek, Sadhana Singh
The Journal of Chemical Physics
Dynamics and Control of Mechanical Systems
article

Non-equilibrium dynamics of disordered bead-spring networks with active forces

Debjyoti Majumdar, Rony Granek, Sadhana Singh
article en

Abstract

We investigate, using Langevin dynamics simulations, the Rouse-type dynamics of active harmonic bead-spring percolation clusters of square and triangular lattices. Two types of active stochastic forces, modeled as a random telegraph process with correlation time τ, are considered: force monopoles, acting on individual nodes in random directions, and force dipoles, where extensile or contractile forces act between pairs of nodes. For force monopoles, a dynamical steady state is reached where the network is dynamically swollen and the mean square displacement (MSD) shows sub-diffusive behavior at t > τ, MSD ∼ tν, with ν=1-ds2 where ds is the spectral dimension, in accord with a previously advanced general analytic theory. In contrast, dipolar forces require diverging times to reach steady state and lead to network shrinkage. Within a quasi-steady-state approximation, the MSD is found to saturate at the same temporal regime t > τ, which is followed by ballistic-like and/or diffusive behaviors. We further extend our study of dipolar forces to dilution regimes above the isostatic threshold, also known as "rigidity percolation". Here, weak dipolar forces effectively do not shrink the network in steady state. Instead, they induce "rotational swimming" of the network. Yet, for the triangular lattice, an incipient discontinuous collapse transition occurs above a critical force amplitude value. Conversely, we find a continuous crossover to a collapsed state for the non-diluted square lattice, resulting from its marginal stability. We suggest that disordered solids be poised above the isostatic point to be stable against active dipolar forces, provided that the dynamical persistent length remains lower than the spring rest length.

The Journal of Chemical PhysicsVol. 163(11)
Ben-Gurion University of the Negev (IL)
Openalex Percentile: Top 69%
Dynamics and Control of Mechanical Systems
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.

Non-equilibrium dynamics of disordered bead-spring networks with active forces — Debjyoti Majumdar, Rony Granek, et al. · The Journal of Chemical Physics (2025) | TGRS Research Map | TGRS