Nonvolatile multistate electrothermal resistive switching in a strongly correlated insulator thin-film device

Strongly correlated insulators, such as Mott or charge-transfer insulators, exhibit a strong temperature dependence in their resistivity. Consequently, self-heating effects can lead to electrothermal instabilities in planar thin-film devices of these materials. When the electrical bias current exceeds a device-specific threshold, the device can switch from a high- to a low-resistance state through the formation of metallic filaments. However, since the filaments are sustained by local Joule heating after they form, reducing the bias current below a second threshold causes them to disappear, returning the device to the high-resistance state. Hence, electrothermal resistive switching is usually volatile. Here, on the contrary, we report on nonvolatile resistive switching in a planar ${\mathrm{Nd}\mathrm{Ni}\mathrm{O}}_{3}$ thin-film device. By combining electrical transport measurements with optical wide-field microscopy, we provide evidence for a metallic filament that persists even after returning the bias current to zero. We attribute this effect to the pronounced hysteresis between the cooling and heating branches in the resistance versus temperature dependence of the device. At least $100$ intermediate resistance states can be prepared, which are persistent as long as the base temperature is kept constant. Further, the switching process is nondestructive, and thermal cycling can reset the device to its pristine state.

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Publication Details

Journal
Physical Review Applied
Published
2025-08-11
DOI
https://doi.org/10.1103/h98b-4438
Citations
2
Primary Topic
Advanced Memory and Neural Computing
Type
article
Field-Weighted Citation Impact
1.46
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article

Nonvolatile multistate electrothermal resistive switching in a strongly correlated insulator thin-film device

Matthias Hepting, Stefan Guénon, Farnaz Tahouni-Bonab, Г. Логвенов et al.
2 citations
Physical Review Applied
Advanced Memory and Neural Computing
1.46
article

Nonvolatile multistate electrothermal resistive switching in a strongly correlated insulator thin-film device

Matthias Hepting, Stefan Guénon, Farnaz Tahouni-Bonab, Г. Логвенов, D. Koelle, R. Kleiner, Theodor Luibrand, B. Keimer, C. Schmid, Georg Cristiani
article en
2 citations

Abstract

Strongly correlated insulators, such as Mott or charge-transfer insulators, exhibit a strong temperature dependence in their resistivity. Consequently, self-heating effects can lead to electrothermal instabilities in planar thin-film devices of these materials. When the electrical bias current exceeds a device-specific threshold, the device can switch from a high- to a low-resistance state through the formation of metallic filaments. However, since the filaments are sustained by local Joule heating after they form, reducing the bias current below a second threshold causes them to disappear, returning the device to the high-resistance state. Hence, electrothermal resistive switching is usually volatile. Here, on the contrary, we report on nonvolatile resistive switching in a planar ${\mathrm{Nd}\mathrm{Ni}\mathrm{O}}_{3}$ thin-film device. By combining electrical transport measurements with optical wide-field microscopy, we provide evidence for a metallic filament that persists even after returning the bias current to zero. We attribute this effect to the pronounced hysteresis between the cooling and heating branches in the resistance versus temperature dependence of the device. At least $100$ intermediate resistance states can be prepared, which are persistent as long as the base temperature is kept constant. Further, the switching process is nondestructive, and thermal cycling can reset the device to its pristine state.

Physical Review AppliedVol. 24(3)
Max Planck Institute for Solid State Research (DE), University of Tübingen (DE)
Openalex Percentile: Top 15%
Advanced Memory and Neural Computing
1.46
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