Demonstration and Frequency Noise Characterization of a 17 µm Quantum Cascade Laser
Abstract The spectral performance of a novel continuous‐wave room‐temperature distributed feedback quantum cascade laser operating is evaluated at the long wavelength of 17 µm. By demonstrating broadband laser absorption spectroscopy of the fundamental vibrational mode of molecules, the spectral range is determined and the spectroscopic potential of this laser is established. The frequency noise is characterized and the line width of this new device is measured, uncovering a discrepancy with the current consensus on the theoretical modeling of quantum cascade lasers. The results confirm the potential of such novel narrow‐line‐width sources for vibrational spectroscopy. Extending laser spectroscopy to longer wavelength is a fascinating prospect that paves the way for a wide range of opportunities from chemical detection, to frequency metrology as well as for exploring light‐matter interaction with an extended variety of molecules, from ultra‐cold diatomic species to increasingly complex molecular systems.
Authors
- T. E. Wall (ORCID: https://orcid.org/0000-0001-6012-0432)
- Mathieu Manceau (ORCID: https://orcid.org/0000-0002-8319-5741)
- R. Teissier (ORCID: https://orcid.org/0000-0002-1453-2433)
- Benoît Darquié (ORCID: https://orcid.org/0000-0002-8623-5817)
- M. R. Tarbutt (ORCID: https://orcid.org/0000-0003-2713-9531)
- А. Н. Баранов (ORCID: https://orcid.org/0000-0003-4940-6098)
- Hadrien Philip
- Olivier Lopez
Institutions
- Centre National de la Recherche Scientifique (FR)
- Université de Montpellier (FR)
- Sorbonne Université (FR)
- Université Sorbonne Paris Nord (FR)
- Laboratoire de physique des lasers (FR)
- Imperial College London (GB)
Publication Details
- Journal
- Laser & Photonics Review
- Published
- 2025-09-05
- DOI
- https://doi.org/10.1002/lpor.202500879
- Primary Topic
- Spectroscopy and Laser Applications
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Imperial College London
- Agence Nationale de la Recherche
- Centre National de la Recherche Scientifique
- FP7 People: Marie-Curie Actions
- HORIZON EUROPE European Research Council