Notable Radiative Effects of Brown Carbon in China Haze
Abstract Brown carbon (BrC), a light‐absorbing organic aerosol, remains poorly constrained in climate models due to unclear sources and formation pathways. In this study, we developed a BrC parameterization scheme by applying multivariate regression to observational data in China, relating BrC concentrations to organic carbon, meteorological conditions, and chemical variables. This scheme was implemented into the WRF‐Chem model to simulate BrC distributions and radiative effects during a haze episode from 1 January–12, 2019. The simulation revealed BrC concentrations ranging from 2.20 to 69.38 μg/m 3 (mean: 11.63 μg/m 3 ), with elevated values in the Beijing‐Tianjin‐Hebei region and Central China. BrC absorption notably decreased surface shortwave radiation by 7.07 W/m 2 and increased atmospheric shortwave radiation by 0.73 W/m 2 , inducing non‐negligible land surface cooling, positive pressure anomalies, and higher near‐surface humidity. These findings underscore the notable radiative influence of BrC in haze‐prone regions of China, with implications for local climate and atmospheric dynamics.
Authors
- Gehui Wang (ORCID: https://orcid.org/0000-0002-0181-4685)
- Luyao Wang (ORCID: https://orcid.org/0000-0002-2403-8156)
- Huizheng Che (ORCID: https://orcid.org/0000-0002-9458-3387)
- Can Wu (ORCID: https://orcid.org/0000-0003-2025-2646)
- Shaojun Lv
- Yubao Chen
- Fanglin Wang (ORCID: https://orcid.org/0009-0009-9378-7394)
- Yanting Lu (ORCID: https://orcid.org/0000-0002-4075-6983)
- Li Li (ORCID: https://orcid.org/0000-0001-5575-0894)
- Lei Zhang (ORCID: https://orcid.org/0000-0001-6268-934X)
- Xingqin An
- Xiaoye Zhang (ORCID: https://orcid.org/0000-0003-2853-9596)
- Yuning Xie (ORCID: https://orcid.org/0000-0002-2255-3357)
Institutions
- Shanghai University (CN)
- China Meteorological Administration (CN)
- Chinese Academy of Meteorological Sciences (CN)
- East China Normal University (CN)
Publication Details
- Journal
- Geophysical Research Letters
- Published
- 2025-09-03
- DOI
- https://doi.org/10.1029/2025gl118037
- Citations
- 1
- Primary Topic
- Atmospheric chemistry and aerosols
- Type
- article
- Field-Weighted Citation Impact
- 1.30
Funders
- National Natural Science Foundation of China
- China Meteorological Administration