Quantum Geometry and the Electric Magnetochiral Anisotropy in Noncentrosymmetric Polar Media

The electric magnetochiral anisotropy is a nonreciprocal phenomenon accessible via second harmonic transport in noncentrosymmetric, time-reversal invariant materials, in which the rectification of current, I, can be controlled by an external magnetic field, B. Quantum geometry, which characterizes the topology of Bloch electrons in a Hilbert space, provides a powerful description of the nonlinear dynamics in topological materials. Here, we demonstrate that the electric magnetochiral anisotropy in noncentrosymmetric polar media owes its existence to the quantum metric, arising from the spin-orbit coupling, and to large Born effective charges. In this context, the reciprocal magnetoresistance βB^{2} is modified to R(I,P,B)=R_{0}[1+βB^{2}+γ^{±}I·(P×B)], where the chirality dependent γ^{±} is determined by the quantum metric dipole and P is the polarization. In 2D, we predict a universal scaling γ^{±}(V)∼V^{-5/2}, which we compare to available phase sensitive, second harmonic transport measurements on hydrothermally grown tellurium films under applied gate voltage, V. The control of rectification by varying I, P, B, and V, demonstrated in this work, opens up new avenues for the building of ultrascaled complementary metal-oxide-semiconductor circuits.

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Publication Details

Journal
Physical Review Letters
Published
2025-09-02
DOI
https://doi.org/10.1103/7nxc-j62y
Citations
1
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
1.25

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article

Quantum Geometry and the Electric Magnetochiral Anisotropy in Noncentrosymmetric Polar Media

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1 citations
Physical Review Letters
Topological Materials and Phenomena
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article

Quantum Geometry and the Electric Magnetochiral Anisotropy in Noncentrosymmetric Polar Media

Pedro V. Lopes, Chang Niu, Pierpaolo Fontana, M. B. Silva Neto, Caio Lewenkopf, Peide D. Ye, Marcus V. O. Moutinho, V.R. Velasco, Kaio E. M. de Souza
article en
1 citations

Abstract

The electric magnetochiral anisotropy is a nonreciprocal phenomenon accessible via second harmonic transport in noncentrosymmetric, time-reversal invariant materials, in which the rectification of current, I, can be controlled by an external magnetic field, B. Quantum geometry, which characterizes the topology of Bloch electrons in a Hilbert space, provides a powerful description of the nonlinear dynamics in topological materials. Here, we demonstrate that the electric magnetochiral anisotropy in noncentrosymmetric polar media owes its existence to the quantum metric, arising from the spin-orbit coupling, and to large Born effective charges. In this context, the reciprocal magnetoresistance βB^{2} is modified to R(I,P,B)=R_{0}[1+βB^{2}+γ^{±}I·(P×B)], where the chirality dependent γ^{±} is determined by the quantum metric dipole and P is the polarization. In 2D, we predict a universal scaling γ^{±}(V)∼V^{-5/2}, which we compare to available phase sensitive, second harmonic transport measurements on hydrothermally grown tellurium films under applied gate voltage, V. The control of rectification by varying I, P, B, and V, demonstrated in this work, opens up new avenues for the building of ultrascaled complementary metal-oxide-semiconductor circuits.

Physical Review LettersVol. 135(10)
Universidade Federal do Rio de Janeiro (BR), Universitat Autònoma de Barcelona (ES), Scuola Internazionale Superiore di Studi Avanzati (IT), Purdue University West Lafayette (US), Universidade Federal do Estado do Rio de Janeiro (BR)
European Commission, Conselho Nacional de Desenvolvimento Científico e Tecnológico, Fundação Carlos Chagas Filho de Amparo à Pesquisa do Estado do Rio de Janeiro, Ministero dell'Università e della Ricerca
Openalex Percentile: Top 18%
Topological Materials and Phenomena
1.25
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