Orbital filtering in edge-state transport of PbSe nanoribbons

Topological insulators are expected to exhibit robust edge-state transport protected by time-reversal symmetry, yet experimental conductance often falls below the quantized limit due to intrinsic and interfacial effects. Here, we demonstrate that the orbital character of topological edge states, governed by spin-orbit coupling and edge termination, plays a critical role in electron injection and transport. Using first-principles calculations combined with nonequilibrium Green's function methods, we investigate PbSe nanoribbons as a model system. We identify an orbital filtering mechanism arising from spin-orbital-entangled edge states, where the $j=1/2$ and $j=3/2$ components of the $p$ orbitals obey symmetry-imposed selection rules at the interface. This effect limits conductance even in the absence of disorder; when present, disorder further promotes an interplay between topological edge states and resonant edge-localized states originating from dangling bonds. Our findings highlight the importance of orbital engineering and angular momentum symmetry mismatch in the design of topological devices and call for an examination of interface physics in quantum materials regarding the topological protection.

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Publication Details

Journal
Physical Review Materials
Published
2025-09-02
DOI
https://doi.org/10.1103/ttfc-9z7d
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
0.00

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article

Orbital filtering in edge-state transport of PbSe nanoribbons

F. Crasto de Lima, A. Fazzio, A. L. Araújo, Carlos Mera Acosta et al.
Physical Review Materials
Topological Materials and Phenomena
article

Orbital filtering in edge-state transport of PbSe nanoribbons

F. Crasto de Lima, A. Fazzio, A. L. Araújo, Carlos Mera Acosta, Rafael L. H. Freire, M. A. Toloza Sandoval
article en

Abstract

Topological insulators are expected to exhibit robust edge-state transport protected by time-reversal symmetry, yet experimental conductance often falls below the quantized limit due to intrinsic and interfacial effects. Here, we demonstrate that the orbital character of topological edge states, governed by spin-orbit coupling and edge termination, plays a critical role in electron injection and transport. Using first-principles calculations combined with nonequilibrium Green's function methods, we investigate PbSe nanoribbons as a model system. We identify an orbital filtering mechanism arising from spin-orbital-entangled edge states, where the $j=1/2$ and $j=3/2$ components of the $p$ orbitals obey symmetry-imposed selection rules at the interface. This effect limits conductance even in the absence of disorder; when present, disorder further promotes an interplay between topological edge states and resonant edge-localized states originating from dangling bonds. Our findings highlight the importance of orbital engineering and angular momentum symmetry mismatch in the design of topological devices and call for an examination of interface physics in quantum materials regarding the topological protection.

Physical Review MaterialsVol. 9(9)
Brazilian Center for Research in Energy and Materials (BR), Universidade Federal do ABC (BR)
Fundação de Amparo à Pesquisa do Estado de São Paulo, Conselho Nacional de Desenvolvimento Científico e Tecnológico, Financiadora de Estudos e Projetos
Openalex Percentile: Top 82%
Topological Materials and Phenomena
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