Nanoengineered Optoexcitonic Switch

The efficiency of most electronic devices is limited by scattering and capacitive losses among purely electronic processes. Charge-neutral excitons could reduce both losses and, thus, offer more efficient switching pathways. However, it remains challenging to achieve exciton transport that is fast, guided, and unidirectional enough for gating processes. We have overcome these obstacles by photonically nanoengineering exciton-photon coupling in a two-dimensional monolayer to create a strong opto-excitonic force capable of driving rapid and long-distance exciton drift transport under ambient conditions. Implementing this strategy, we have demonstrated an optoexcitonic switch along a one-dimensional (1D) exciton guide, with gating performance already rivaling that of state-of-the-art electronic switches. Our work establishes the basis for room-temperature implementation of opto-excitonic circuits.

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Publication Details

Journal
ACS Nano
Published
2025-09-01
DOI
https://doi.org/10.1021/acsnano.5c05057
Primary Topic
Neural Networks and Reservoir Computing
Type
article
Field-Weighted Citation Impact
0.00

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article

Nanoengineered Optoexcitonic Switch

Zidong Li, Parag B. Deotare, Zhaohan Jiang, M. Kira et al.
5 links
ACS Nano
Neural Networks and Reservoir Computing
article

Nanoengineered Optoexcitonic Switch

Zidong Li, Parag B. Deotare, Zhaohan Jiang, M. Kira, Kanak Datta, Matthias Florian
article en

Abstract

The efficiency of most electronic devices is limited by scattering and capacitive losses among purely electronic processes. Charge-neutral excitons could reduce both losses and, thus, offer more efficient switching pathways. However, it remains challenging to achieve exciton transport that is fast, guided, and unidirectional enough for gating processes. We have overcome these obstacles by photonically nanoengineering exciton-photon coupling in a two-dimensional monolayer to create a strong opto-excitonic force capable of driving rapid and long-distance exciton drift transport under ambient conditions. Implementing this strategy, we have demonstrated an optoexcitonic switch along a one-dimensional (1D) exciton guide, with gating performance already rivaling that of state-of-the-art electronic switches. Our work establishes the basis for room-temperature implementation of opto-excitonic circuits.

ACS NanoVol. 19(36)
University of Michigan (US), Michigan Medicine (US), Quantum Chemistry Research Institute (JP), Ann Arbor Center for Independent Living (US), Quantum Signal (United States) (US)
National Science Foundation, Air Force Office of Scientific Research, Army Research Office
Openalex Percentile: Top 88%
Neural Networks and Reservoir Computing
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Nanoengineered Optoexcitonic Switch — Zidong Li, Parag B. Deotare, et al. · ACS Nano (2025) | TGRS Research Map | TGRS