Tailoring directional emission of colloidal quantum dots <i>via</i> mode coupling with photonic crystals

Precise control over the emission direction of colloidal quantum dots (CQDs), which are promising color conversion materials for micro-light-emitting-diode displays, is increasingly important for augmented-reality and virtual-reality near-eye optics. Here, we report a fully dielectric silicon nitride (Si<sub>3</sub>N<sub>4</sub>) photonic crystal (PhC) platform that boosts CQD photoluminescence by an 8.5-fold increase while compressing the angular full-width at half-maximum to 6.5°. Embedding CdSe/ZnS CQDs into one- and two-dimensional PhCs aligns band-edge guided-mode resonances with the emitter spectrum, converting guided Bloch modes into leaky modes that satisfy in-plane phase-matching conditions. Finite-difference time-domain simulations, photonic-band mapping, and angle-resolved photoluminescence measurements confirm that the PhC period deterministically sets the emission angle and that the PhC lattice funnels light symmetrically around the Γ point to achieve omnidirectional collimation. This all-dielectric architecture offers intrinsically low propagation loss and provides a scalable, lithography-defined platform for bright, color-pure, and angularly engineered light sources for next-generation displays, sensors, and on-chip photonic devices.

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Publication Details

Journal
Nanoscale
Published
2025-01-01
DOI
https://doi.org/10.1039/d5nr02616d
Primary Topic
Photonic Crystals and Applications
Type
article
Field-Weighted Citation Impact
0.00

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article

Tailoring directional emission of colloidal quantum dots via mode coupling with photonic crystals

Gregorio Baek, Sehyeon Park, Sunwoo Woo, M.C. Lee et al.
Nanoscale
Photonic Crystals and Applications
article

Tailoring directional emission of colloidal quantum dots via mode coupling with photonic crystals

Gregorio Baek, Sehyeon Park, Sunwoo Woo, M.C. Lee, Young-Jun Chung, J.M. Min
article en

Abstract

Precise control over the emission direction of colloidal quantum dots (CQDs), which are promising color conversion materials for micro-light-emitting-diode displays, is increasingly important for augmented-reality and virtual-reality near-eye optics. Here, we report a fully dielectric silicon nitride (Si<sub>3</sub>N<sub>4</sub>) photonic crystal (PhC) platform that boosts CQD photoluminescence by an 8.5-fold increase while compressing the angular full-width at half-maximum to 6.5°. Embedding CdSe/ZnS CQDs into one- and two-dimensional PhCs aligns band-edge guided-mode resonances with the emitter spectrum, converting guided Bloch modes into leaky modes that satisfy in-plane phase-matching conditions. Finite-difference time-domain simulations, photonic-band mapping, and angle-resolved photoluminescence measurements confirm that the PhC period deterministically sets the emission angle and that the PhC lattice funnels light symmetrically around the Γ point to achieve omnidirectional collimation. This all-dielectric architecture offers intrinsically low propagation loss and provides a scalable, lithography-defined platform for bright, color-pure, and angularly engineered light sources for next-generation displays, sensors, and on-chip photonic devices.

NanoscaleVol. 17(36)
Seoul National University (KR)
Seoul National University, Ministry of Trade, Industry and Energy, Ministry of Science and ICT, South Korea
Openalex Percentile: Top 82%
Photonic Crystals and Applications
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Tailoring directional emission of colloidal quantum dots <i>via</i> mode coupling with photonic crystals — Gregorio Baek, Sehyeon Park, et al. · Nanoscale (2025) | TGRS Research Map | TGRS