Tailoring directional emission of colloidal quantum dots <i>via</i> mode coupling with photonic crystals
Precise control over the emission direction of colloidal quantum dots (CQDs), which are promising color conversion materials for micro-light-emitting-diode displays, is increasingly important for augmented-reality and virtual-reality near-eye optics. Here, we report a fully dielectric silicon nitride (Si<sub>3</sub>N<sub>4</sub>) photonic crystal (PhC) platform that boosts CQD photoluminescence by an 8.5-fold increase while compressing the angular full-width at half-maximum to 6.5°. Embedding CdSe/ZnS CQDs into one- and two-dimensional PhCs aligns band-edge guided-mode resonances with the emitter spectrum, converting guided Bloch modes into leaky modes that satisfy in-plane phase-matching conditions. Finite-difference time-domain simulations, photonic-band mapping, and angle-resolved photoluminescence measurements confirm that the PhC period deterministically sets the emission angle and that the PhC lattice funnels light symmetrically around the Γ point to achieve omnidirectional collimation. This all-dielectric architecture offers intrinsically low propagation loss and provides a scalable, lithography-defined platform for bright, color-pure, and angularly engineered light sources for next-generation displays, sensors, and on-chip photonic devices.
Authors
- Gregorio Baek
- Sehyeon Park
- Sunwoo Woo (ORCID: https://orcid.org/0000-0003-1023-6669)
- M.C. Lee (ORCID: https://orcid.org/0009-0007-1256-4267)
- Young-Jun Chung (ORCID: https://orcid.org/0009-0000-4495-631X)
- J.M. Min
Institutions
- Seoul National University (KR)
Publication Details
- Journal
- Nanoscale
- Published
- 2025-01-01
- DOI
- https://doi.org/10.1039/d5nr02616d
- Primary Topic
- Photonic Crystals and Applications
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Seoul National University
- Ministry of Trade, Industry and Energy
- Ministry of Science and ICT, South Korea