Enhanced Radiation Tolerance of MoS<sub>2</sub> FET via Al<sub>2</sub>O<sub>3</sub> Insertion on SiO<sub>2</sub> Dielectric

Molybdenum disulfide (MoS2) combines a tunable bandgap and high carrier mobility, making it promising for nanoelectronics. Its inherent radiation tolerance further promotes the development of radiation-hardened devices for extreme environments, such as outer space exploration. Although research has been conducted on the damage mechanisms of MoS2 field-effect transistors (FETs) under ionizing irradiation, studies on the modulation of charge trapping through gate dielectric engineering to enhance their radiation tolerance remain relatively scarce. In this work, we designed back-gated MoS2 FETs by inserting a traditional high-κ dielectric alumina (Al2O3) between the MoS2 and silicon dioxide (SiO2), forming a MoS2/Al2O3/SiO2 structure, and compared them with MoS2/SiO2 FETs. The devices were subjected to 200 keV proton irradiation at a dose of 1 × 1014 cm–2, and the comparative results show that the MoS2 FET with Al2O3 exhibits significantly enhanced radiation tolerance. This improvement is primarily attributed to the high dielectric screening effect of Al2O3, which greatly reduces Coulomb scattering, thereby not only mitigating displacement damage in the MoS2 channel but also effectively suppressing the generation of interface and oxide trapped charges. Therefore, dielectric engineering serves as a critical strategy to provide support for the development of two-dimensional electronic systems that can operate reliably in extreme radiation environments.

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Publication Details

Journal
The Journal of Physical Chemistry C
Published
2025-08-28
DOI
https://doi.org/10.1021/acs.jpcc.5c04658
Primary Topic
2D Materials and Applications
Type
article
Field-Weighted Citation Impact
0.00

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article

Enhanced Radiation Tolerance of MoS2 FET via Al2O3 Insertion on SiO2 Dielectric

Ting-Qing Liao, Chih‐Wei Luo, Changzhong Jiang, Wenjing Qin et al.
5 links
The Journal of Physical Chemistry C
2D Materials and Applications
article

Enhanced Radiation Tolerance of MoS2 FET via Al2O3 Insertion on SiO2 Dielectric

Ting-Qing Liao, Chih‐Wei Luo, Changzhong Jiang, Wenjing Qin, Sung Chun Chen, Zhaozhao Yang
article en

Abstract

Molybdenum disulfide (MoS2) combines a tunable bandgap and high carrier mobility, making it promising for nanoelectronics. Its inherent radiation tolerance further promotes the development of radiation-hardened devices for extreme environments, such as outer space exploration. Although research has been conducted on the damage mechanisms of MoS2 field-effect transistors (FETs) under ionizing irradiation, studies on the modulation of charge trapping through gate dielectric engineering to enhance their radiation tolerance remain relatively scarce. In this work, we designed back-gated MoS2 FETs by inserting a traditional high-κ dielectric alumina (Al2O3) between the MoS2 and silicon dioxide (SiO2), forming a MoS2/Al2O3/SiO2 structure, and compared them with MoS2/SiO2 FETs. The devices were subjected to 200 keV proton irradiation at a dose of 1 × 1014 cm–2, and the comparative results show that the MoS2 FET with Al2O3 exhibits significantly enhanced radiation tolerance. This improvement is primarily attributed to the high dielectric screening effect of Al2O3, which greatly reduces Coulomb scattering, thereby not only mitigating displacement damage in the MoS2 channel but also effectively suppressing the generation of interface and oxide trapped charges. Therefore, dielectric engineering serves as a critical strategy to provide support for the development of two-dimensional electronic systems that can operate reliably in extreme radiation environments.

The Journal of Physical Chemistry CVol. 129(36)
Hunan University (CN), Hunan Normal University (CN), Beijing Zhongke Science and Technology (China) (CN), Division of Materials Science and Engineering (AU), Quantum Technologies (Sweden) (SE)
Education Department of Hunan Province, Hunan Normal University
Affordable and clean energy
Openalex Percentile: Top 83%
2D Materials and Applications
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