Electrical Control of Ultrafast Magnetic Speeds in Graphene Spin Field-Effect Junctions

We demonstrate ultrafast graphene spin-field-effect junctions, where gate-tunable superdiffusive spin currents across graphene-ferromagnet interfaces enable electric field control of magnetization dynamics in the ferromagnet. By electrostatically tuning the Fermi level in graphene underlying a cobalt thin film, we modulate the ultrafast spin transport across graphene-cobalt interfaces, reducing femtosecond laser-induced demagnetization time from 203 fs in bare cobalt thin films to 93 fs, a more than 100% increase in the rate of magnetization quenching. Supported by superdiffusive spin transport calculations, our findings unlock field-tunable magnetic speeds in devices, paving the way for innovations in subpicosecond spintronic memory-logic operations. Furthermore, this work creates new possibilities for electrical modulation of spin dynamics and ultrafast spin injection into two-dimensional quantum materials, with potential for next-generation quantum sensors and faster magnetic technologies.

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Publication Details

Journal
Physical Review Letters
Published
2025-08-28
DOI
https://doi.org/10.1103/7ldk-csp9
Primary Topic
Magnetic properties of thin films
Type
article
Field-Weighted Citation Impact
0.00

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article

Electrical Control of Ultrafast Magnetic Speeds in Graphene Spin Field-Effect Junctions

Olof Karis, Anjan Barman, Francesco Foggetti, Suchetana Mukhopadhyay et al.
Physical Review Letters
Magnetic properties of thin films
article

Electrical Control of Ultrafast Magnetic Speeds in Graphene Spin Field-Effect Junctions

Olof Karis, Anjan Barman, Francesco Foggetti, Suchetana Mukhopadhyay, M. Venkata Kamalakar, Peter M. Oppeneer, David Muradas-Belinchón, Surya N. Panda
article en

Abstract

We demonstrate ultrafast graphene spin-field-effect junctions, where gate-tunable superdiffusive spin currents across graphene-ferromagnet interfaces enable electric field control of magnetization dynamics in the ferromagnet. By electrostatically tuning the Fermi level in graphene underlying a cobalt thin film, we modulate the ultrafast spin transport across graphene-cobalt interfaces, reducing femtosecond laser-induced demagnetization time from 203 fs in bare cobalt thin films to 93 fs, a more than 100% increase in the rate of magnetization quenching. Supported by superdiffusive spin transport calculations, our findings unlock field-tunable magnetic speeds in devices, paving the way for innovations in subpicosecond spintronic memory-logic operations. Furthermore, this work creates new possibilities for electrical modulation of spin dynamics and ultrafast spin injection into two-dimensional quantum materials, with potential for next-generation quantum sensors and faster magnetic technologies.

Physical Review LettersVol. 135(9)
Uppsala University (SE), Indian Institute of Science Education and Research Kolkata (IN), Bose (United States) (US), S.N. Bose National Centre for Basic Sciences (IN)
Department of Science and Technology, Ministry of Science and Technology, India, National Science Council, Knut och Alice Wallenbergs Stiftelse, Stiftelsen Olle Engkvist Byggmästare, Vetenskapsrådet, European Research Council, S. N. Bose National Centre for Basic Sciences
Openalex Percentile: Top 83%
Magnetic properties of thin films
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