Incoherent Measurement of a Sub-10 kHz Optical Linewidth

Quantum state lifetimes T_{2}, or equivalently homogeneous linewidths Γ_{h}=1/πT_{2}, are a key parameter for understanding decoherence processes in quantum systems and assessing their potential for applications in quantum technologies. The most common tool for measuring narrow optical homogeneous linewidths, i.e., long T_{2}, is the measurement of coherent photon echo emissions, which however gives very weak signal when the number of emitters is small. This strongly hampers the development of nanomaterials, such as those based on rare earth ions, for quantum communication and processing. In this work, we propose, and demonstrate in an erbium doped crystal, a measurement of photon echoes based on incoherent fluorescence detection and its variance analysis. It gives access to T_{2} through a much larger signal than direct photon echo detection, and, importantly, with a laser which is incoherent over the measurement timescale, on the order of a few T_{2}. Our results thus open the way to efficiently assess the properties of a broad range of emitters and materials for applications in quantum nanophotonics.

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Publication Details

Journal
Physical Review Letters
Published
2025-08-26
DOI
https://doi.org/10.1103/xkp5-v9m8
Primary Topic
Photonic and Optical Devices
Type
article
Field-Weighted Citation Impact
0.00

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article

Incoherent Measurement of a Sub-10 kHz Optical Linewidth

Alexey Tiranov, Patrice Bertet, Philippe Goldner, Diana Serrano et al.
Physical Review Letters
Photonic and Optical Devices
article

Incoherent Measurement of a Sub-10 kHz Optical Linewidth

Alexey Tiranov, Patrice Bertet, Philippe Goldner, Diana Serrano, Emmanuel Flurin, Félix Montjovet-Basset, Jayash Panigrahi, Alban Ferrier
article en

Abstract

Quantum state lifetimes T_{2}, or equivalently homogeneous linewidths Γ_{h}=1/πT_{2}, are a key parameter for understanding decoherence processes in quantum systems and assessing their potential for applications in quantum technologies. The most common tool for measuring narrow optical homogeneous linewidths, i.e., long T_{2}, is the measurement of coherent photon echo emissions, which however gives very weak signal when the number of emitters is small. This strongly hampers the development of nanomaterials, such as those based on rare earth ions, for quantum communication and processing. In this work, we propose, and demonstrate in an erbium doped crystal, a measurement of photon echoes based on incoherent fluorescence detection and its variance analysis. It gives access to T_{2} through a much larger signal than direct photon echo detection, and, importantly, with a laser which is incoherent over the measurement timescale, on the order of a few T_{2}. Our results thus open the way to efficiently assess the properties of a broad range of emitters and materials for applications in quantum nanophotonics.

Physical Review LettersVol. 135(9)
Centre National de la Recherche Scientifique (FR), Chimie ParisTech - PSL (FR), Université Paris Sciences et Lettres (FR), Université Paris-Saclay (FR), Sorbonne Université (FR), Institut de Recherche de Chimie Paris (FR), Laboratoire Médiations (FR)
Agence Nationale de la Recherche, Horizon 2020 Framework Programme, European Research Council
Affordable and clean energy
Openalex Percentile: Top 79%
Photonic and Optical Devices
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