SOH estimation for lithium-ion batteries using the distribution of relaxation time and feature optimized multilayer perceptron

Electrochemical impedance spectroscopy (EIS) offers abundant dynamic information related to battery degradation. However, the distribution of relaxation time (DRT) methods often produces ambiguous timescale features due to overlapping peaks and the subjective selection of regularization parameters. We propose a DRT method based on RQ elements. This approach significantly reduces parameter sensitivity and enhances the stability of extracted features. The most informative peaks and their combinations are optimized using a feature selection algorithm and are then used as inputs to a multilayer perceptron (MLP) for SOH estimation. The proposed method is validated on two commercial LIB chemistries under different states of charge (SOC) as well as on an open-access dataset. The results demonstrate that the health indicators extracted via the RQ-DRT method and feature combinations effectively reduce redundancy and improve SOH estimation performance. By bridging impedance-based timescale analysis and machine learning, this work provides a practical pathway for SOH monitoring in battery management systems.

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Publication Details

Journal
iScience
Published
2025-08-26
DOI
https://doi.org/10.1016/j.isci.2025.113443
Primary Topic
Advanced Battery Technologies Research
Type
article
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article

SOH estimation for lithium-ion batteries using the distribution of relaxation time and feature optimized multilayer perceptron

Shiqiang Liu, Xiaole Ma, Qi Zhang, Xiaoqian Dai et al.
iScience
Advanced Battery Technologies Research
article

SOH estimation for lithium-ion batteries using the distribution of relaxation time and feature optimized multilayer perceptron

Shiqiang Liu, Xiaole Ma, Qi Zhang, Xiaoqian Dai, Dafang Wang, Fang Wang, Shiqin Chen
article en

Abstract

Electrochemical impedance spectroscopy (EIS) offers abundant dynamic information related to battery degradation. However, the distribution of relaxation time (DRT) methods often produces ambiguous timescale features due to overlapping peaks and the subjective selection of regularization parameters. We propose a DRT method based on RQ elements. This approach significantly reduces parameter sensitivity and enhances the stability of extracted features. The most informative peaks and their combinations are optimized using a feature selection algorithm and are then used as inputs to a multilayer perceptron (MLP) for SOH estimation. The proposed method is validated on two commercial LIB chemistries under different states of charge (SOC) as well as on an open-access dataset. The results demonstrate that the health indicators extracted via the RQ-DRT method and feature combinations effectively reduce redundancy and improve SOH estimation performance. By bridging impedance-based timescale analysis and machine learning, this work provides a practical pathway for SOH monitoring in battery management systems.

iScienceVol. 28(9)
Harbin Institute of Technology (CN), China Automotive Technology and Research Center (CN)
Affordable and clean energy
Openalex Percentile: Top 76%
Advanced Battery Technologies Research
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