Preheating applied on a 915 MHz CO2 microwave plasma: Unlocking the potential for heat recycling in plasma systems

We investigated the effects of inlet gas preheating on plasma performance in a vortex-stabilized 915 MHz CO 2 microwave plasma reactor. Spatially resolved spectroscopic measurements of the plasma were employed to understand how preheating affects the temperature profile. Thermographic measurements of the reaction chamber analyzed losses through the wall, offering deeper insights into the thermal changes within the system. The overall conversion performance was evaluated using gas chromatography. We demonstrate that recycling less than 10 % of the input power to preheat CO 2 ( T inlet = 700 K) can increase the energy efficiency of CO 2 conversion by up to 1.7 times at conditions near atmospheric pressure (700 mbar), at moderate microwave power (1132 W). The results indicate that preheating affects plasma fluid dynamics, resulting in shifts in plasma contraction and increased spatial temperature profile, or reactive volume, with higher inlet temperatures. This study provides new insights into the potential of integrating heat recycling in plasma reactors for future industrial applications. • Preheating the input gas of a CO 2 microwave plasma improves conversion and efficiency. • Preheating the input flow alters flow and contraction dynamics • Increased conversion is due to an enlargement of the productive ‘reactive volume’.

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Publication Details

Journal
Chemical Engineering Journal
Published
2025-08-26
DOI
https://doi.org/10.1016/j.cej.2025.167294
Citations
2
Primary Topic
Plasma Applications and Diagnostics
Type
article
Field-Weighted Citation Impact
2.72

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article

Preheating applied on a 915 MHz CO2 microwave plasma: Unlocking the potential for heat recycling in plasma systems

Elizabeth Rose Mercer, W.A. Bongers, F J J Peeters, Annemie Bogaerts et al.
2 citations
Chemical Engineering Journal
Plasma Applications and Diagnostics
2.72
article

Preheating applied on a 915 MHz CO2 microwave plasma: Unlocking the potential for heat recycling in plasma systems

Elizabeth Rose Mercer, W.A. Bongers, F J J Peeters, Annemie Bogaerts, F.M.A. Smits, C.F.A.M. van Deursen, M. C. M. van de Sanden
article en
2 citations

Abstract

We investigated the effects of inlet gas preheating on plasma performance in a vortex-stabilized 915 MHz CO 2 microwave plasma reactor. Spatially resolved spectroscopic measurements of the plasma were employed to understand how preheating affects the temperature profile. Thermographic measurements of the reaction chamber analyzed losses through the wall, offering deeper insights into the thermal changes within the system. The overall conversion performance was evaluated using gas chromatography. We demonstrate that recycling less than 10 % of the input power to preheat CO 2 ( T inlet = 700 K) can increase the energy efficiency of CO 2 conversion by up to 1.7 times at conditions near atmospheric pressure (700 mbar), at moderate microwave power (1132 W). The results indicate that preheating affects plasma fluid dynamics, resulting in shifts in plasma contraction and increased spatial temperature profile, or reactive volume, with higher inlet temperatures. This study provides new insights into the potential of integrating heat recycling in plasma reactors for future industrial applications. • Preheating the input gas of a CO 2 microwave plasma improves conversion and efficiency. • Preheating the input flow alters flow and contraction dynamics • Increased conversion is due to an enlargement of the productive ‘reactive volume’.

Chemical Engineering JournalVol. 522
Rijksmuseum (NL), University of Antwerp (BE), Fontys University of Applied Sciences (NL), Maritime Research Institute Netherlands (NL), Dutch Institute for Fundamental Energy Research (NL), Eindhoven University of Technology (NL)
European Commission, Nederlandse Organisatie voor Wetenschappelijk Onderzoek
Openalex Percentile: Top 9%
Plasma Applications and Diagnostics
2.72
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