Towards a global phase diagram of Ce-based dipolar-octupolar pyrochlore magnets under magnetic fields

Ce-based dipolar-octupolar pyrochlores have emerged as leading candidates for realizing the elusive $\ensuremath{\pi}$-flux quantum spin ice, yet a definitive identification remains unsettled. The authors establish here a global magnetic field tuned phase diagram for Ce${}_{2}$(Zr,Sn,Hf)${}_{2}$O${}_{7}$, using gauge mean-field theory. Distinctive field direction dependent responses---ranging from critical fields differing by an order of magnitude, to split multi-peak dynamical spectra, to contrasting magnetostriction profiles---reveal powerful probes of the system's underlying multipolar nature. These predictions provide a concrete roadmap for neutron scattering and thermodynamic experiments.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-08-26
DOI
https://doi.org/10.1103/8mhy-qwsw
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
0.00

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article

Towards a global phase diagram of Ce-based dipolar-octupolar pyrochlore magnets under magnetic fields

Yong Baek Kim, Zhengbang Zhou
Physical review. B./Physical review. B
Advanced Condensed Matter Physics
article

Towards a global phase diagram of Ce-based dipolar-octupolar pyrochlore magnets under magnetic fields

Yong Baek Kim, Zhengbang Zhou
article en

Abstract

Ce-based dipolar-octupolar pyrochlores have emerged as leading candidates for realizing the elusive $\ensuremath{\pi}$-flux quantum spin ice, yet a definitive identification remains unsettled. The authors establish here a global magnetic field tuned phase diagram for Ce${}_{2}$(Zr,Sn,Hf)${}_{2}$O${}_{7}$, using gauge mean-field theory. Distinctive field direction dependent responses---ranging from critical fields differing by an order of magnitude, to split multi-peak dynamical spectra, to contrasting magnetostriction profiles---reveal powerful probes of the system's underlying multipolar nature. These predictions provide a concrete roadmap for neutron scattering and thermodynamic experiments.

Physical review. B./Physical review. BVol. 112(6)
University of Toronto (CA)
Natural Sciences and Engineering Research Council of Canada
Openalex Percentile: Top 86%
Advanced Condensed Matter Physics
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