Observation of Persistent Zero Modes and Superconducting Vortex Doublets in UTe<sub>2</sub>
Superconducting vortices can reveal electron pairing details and nucleate topologically protected states. Yet, vortices of bulk spin-triplet superconductors have never been visualized at the atomic scale. Recently, UTe<sub>2</sub> has emerged as a prime spin-triplet superconductor, but its superconducting order parameter is elusive, and whether time-reversal symmetry (TRS) is broken remains unsettled. Here, we visualize vortices on the (011) surface of ultraclean UTe<sub>2</sub> single crystals (<i>T</i><sub>c</sub> = 2.1 K) using scanning tunneling microscopy (STM). We introduce <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mfrac><mml:mrow><mml:msup><mml:mi>d</mml:mi><mml:mn>2</mml:mn></mml:msup><mml:mi>I</mml:mi></mml:mrow><mml:mrow><mml:mi>d</mml:mi><mml:msup><mml:mi>V</mml:mi><mml:mn>2</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:math> imaging as an effective technique for vortex visualization in superconductors with substantial residual zero-energy density of states (DOS), as in UTe<sub>2</sub>. Anisotropic single-flux-quantum vortices, with coherence lengths of ∼12 nm (4 nm) parallel (perpendicular) to the <b>a</b>-axis, form a triangular vortex lattice (VL) under a small out-of-plane magnetic field. The invariance of vortex structures and VL under changes of field polarity and cooling history strongly supports time-reversal invariant superconductivity under zero field. At vortex cores (VCs), nonsplit, spectrally sharp zero-bias conductance peaks (ZBPs) persist up 8 T that are consistent with symmetry-protected Majorana zero modes (MZMs) in a topological vortex line. Close examination of vortex structures reveals a mirror-asymmetric doublet─one with ZBPs and another with an enhanced apparent gap, possibly originating from a field-induced multicomponent order parameter.
Authors
- Mitchell M. Bordelon (ORCID: https://orcid.org/0000-0001-5611-5315)
- Fang-Jun Cheng
- J. Douglas McKenzie (ORCID: https://orcid.org/0000-0003-3700-4577)
- P. F. S. Rosa (ORCID: https://orcid.org/0000-0002-3437-548X)
- Yi‐Ting Hsu (ORCID: https://orcid.org/0000-0002-6340-8404)
- S. M. Thomas (ORCID: https://orcid.org/0000-0003-0889-4435)
- Matthew Toole
- Xiaolong Liu (ORCID: https://orcid.org/0000-0002-6186-5257)
- Nileema Sharma (ORCID: https://orcid.org/0009-0005-7513-3363)
Institutions
- University of Notre Dame (US)
- Los Alamos National Laboratory (US)
Publication Details
- Journal
- ACS Nano
- Published
- 2025-08-26
- DOI
- https://doi.org/10.1021/acsnano.5c08406
- Citations
- 4
- Primary Topic
- Rare-earth and actinide compounds
- Type
- article
- Field-Weighted Citation Impact
- 5.03
Funders
- University of Notre Dame
- Office of Science
- Division of Materials Research
- Basic Energy Sciences