Observation of Persistent Zero Modes and Superconducting Vortex Doublets in UTe<sub>2</sub>

Superconducting vortices can reveal electron pairing details and nucleate topologically protected states. Yet, vortices of bulk spin-triplet superconductors have never been visualized at the atomic scale. Recently, UTe<sub>2</sub> has emerged as a prime spin-triplet superconductor, but its superconducting order parameter is elusive, and whether time-reversal symmetry (TRS) is broken remains unsettled. Here, we visualize vortices on the (011) surface of ultraclean UTe<sub>2</sub> single crystals (<i>T</i><sub>c</sub> = 2.1 K) using scanning tunneling microscopy (STM). We introduce <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mfrac><mml:mrow><mml:msup><mml:mi>d</mml:mi><mml:mn>2</mml:mn></mml:msup><mml:mi>I</mml:mi></mml:mrow><mml:mrow><mml:mi>d</mml:mi><mml:msup><mml:mi>V</mml:mi><mml:mn>2</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:math> imaging as an effective technique for vortex visualization in superconductors with substantial residual zero-energy density of states (DOS), as in UTe<sub>2</sub>. Anisotropic single-flux-quantum vortices, with coherence lengths of ∼12 nm (4 nm) parallel (perpendicular) to the <b>a</b>-axis, form a triangular vortex lattice (VL) under a small out-of-plane magnetic field. The invariance of vortex structures and VL under changes of field polarity and cooling history strongly supports time-reversal invariant superconductivity under zero field. At vortex cores (VCs), nonsplit, spectrally sharp zero-bias conductance peaks (ZBPs) persist up 8 T that are consistent with symmetry-protected Majorana zero modes (MZMs) in a topological vortex line. Close examination of vortex structures reveals a mirror-asymmetric doublet─one with ZBPs and another with an enhanced apparent gap, possibly originating from a field-induced multicomponent order parameter.

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Publication Details

Journal
ACS Nano
Published
2025-08-26
DOI
https://doi.org/10.1021/acsnano.5c08406
Citations
4
Primary Topic
Rare-earth and actinide compounds
Type
article
Field-Weighted Citation Impact
5.03

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article

Observation of Persistent Zero Modes and Superconducting Vortex Doublets in UTe2

Mitchell M. Bordelon, Fang-Jun Cheng, J. Douglas McKenzie, P. F. S. Rosa et al.
4 citations
ACS Nano
Rare-earth and actinide compounds
5.03
article

Observation of Persistent Zero Modes and Superconducting Vortex Doublets in UTe2

Mitchell M. Bordelon, Fang-Jun Cheng, J. Douglas McKenzie, P. F. S. Rosa, Yi‐Ting Hsu, S. M. Thomas, Matthew Toole, Xiaolong Liu, Nileema Sharma
article en
4 citations

Abstract

Superconducting vortices can reveal electron pairing details and nucleate topologically protected states. Yet, vortices of bulk spin-triplet superconductors have never been visualized at the atomic scale. Recently, UTe<sub>2</sub> has emerged as a prime spin-triplet superconductor, but its superconducting order parameter is elusive, and whether time-reversal symmetry (TRS) is broken remains unsettled. Here, we visualize vortices on the (011) surface of ultraclean UTe<sub>2</sub> single crystals (<i>T</i><sub>c</sub> = 2.1 K) using scanning tunneling microscopy (STM). We introduce <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mfrac><mml:mrow><mml:msup><mml:mi>d</mml:mi><mml:mn>2</mml:mn></mml:msup><mml:mi>I</mml:mi></mml:mrow><mml:mrow><mml:mi>d</mml:mi><mml:msup><mml:mi>V</mml:mi><mml:mn>2</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:math> imaging as an effective technique for vortex visualization in superconductors with substantial residual zero-energy density of states (DOS), as in UTe<sub>2</sub>. Anisotropic single-flux-quantum vortices, with coherence lengths of ∼12 nm (4 nm) parallel (perpendicular) to the <b>a</b>-axis, form a triangular vortex lattice (VL) under a small out-of-plane magnetic field. The invariance of vortex structures and VL under changes of field polarity and cooling history strongly supports time-reversal invariant superconductivity under zero field. At vortex cores (VCs), nonsplit, spectrally sharp zero-bias conductance peaks (ZBPs) persist up 8 T that are consistent with symmetry-protected Majorana zero modes (MZMs) in a topological vortex line. Close examination of vortex structures reveals a mirror-asymmetric doublet─one with ZBPs and another with an enhanced apparent gap, possibly originating from a field-induced multicomponent order parameter.

ACS NanoVol. 19(35)
University of Notre Dame (US), Los Alamos National Laboratory (US)
University of Notre Dame, Office of Science, Division of Materials Research, Basic Energy Sciences
Climate action
Openalex Percentile: Top 5%
Rare-earth and actinide compounds
5.03
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